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Electronic and ionic conduction in ligand-free lead selenide colloidal quantum dots
Results in Physics ( IF 4.4 ) Pub Date : 2020-04-17 , DOI: 10.1016/j.rinp.2020.103113
Byoungnam Park

We fabricated a ligand-free lead selenide (PbSe) colloidal quantum dot (CQD) film and probed its electrical properties using a field-effect transistor (FET) at low temperature. The contribution of the ionic conduction to the electrical properties in the PbSe CQD film became significant after ligand removal using ammonium sulfide [(NH4)2S], evidenced by temperature-dependent FET mobility, threshold voltage, and current hysteresis depending on gate scan direction. The enhanced FET mobility and increased carrier concentration at a lower temperature are attributed to reduced ionic conduction, suppressing the gate electric field screening at the PbSe/SiO2 interface.



中文翻译:

无配体硒化铅胶体量子点中的电子和离子传导

我们制造了无配体硒化铅(PbSe)胶体量子点(CQD)膜,并在低温下使用场效应晶体管(FET)探测了其电性能。在使用硫化铵[(NH 42 S]去除配体后,离子传导对PbSe CQD膜中电性能的贡献变得显着,这取决于温度依赖的FET迁移率,阈值电压和取决于门扫描的电流滞后方向。较低的温度下增强的FET迁移率和增加的载流子浓度归因于离子传导的减少,从而抑制了PbSe / SiO 2界面处的栅电场屏蔽。

更新日期:2020-04-17
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