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Optimized Metal Chalcogenides for Boosting Water Splitting.
Advanced Science ( IF 14.3 ) Pub Date : 2020-04-06 , DOI: 10.1002/advs.201903070
Jie Yin 1, 2 , Jing Jin 1 , Honghong Lin 2 , Zhouyang Yin 2 , Jianyi Li 1 , Min Lu 1 , Linchuan Guo 1 , Pinxian Xi 1 , Yu Tang 1 , Chun-Hua Yan 1
Affiliation  

Electrocatalytic water splitting (2H2O → 2H2 + O2) is a very promising avenue to effectively and environmentally friendly produce highly pure hydrogen (H2) and oxygen (O2) at a large scale. Different materials have been developed to enhance the efficiency for water splitting. Among them, chalcogenides with unique atomic arrangement and high electronic transport show interesting catalytic properties in various electrochemical reactions, such as the hydrogen evolution reaction, oxygen evolution reaction, and overall water splitting, while the control of their morphology and structure is of vital importance to their catalytic performance. Herein, the general synthetic methods are summarized to prepare metal chalcogenides and different strategies are designed to improve their catalytic performance for water splitting. The remaining challenges in the research and development of metal chalcogenides and possible directions for future research are also summarized.

中文翻译:

用于促进水分解的优化金属硫属化物。

电催化水分解(2H2O → 2H2 + O2)是一种非常有前景的有效且环保地大规模生产高纯氢气(H2)和氧气(O2)的途径。已经开发出不同的材料来提高水分解的效率。其中,具有独特原子排列和高电子传输的硫族化物在各种电化学反应中表现出有趣的催化性能,例如析氢反应、析氧反应和整体水分解,而其形貌和结构的控制对于催化化学反应至关重要。它们的催化性能。在此,总结了制备金属硫属化物的一般合成方法,并设计了不同的策略来提高其水分解催化性能。还总结了金属硫属化物研究和开发中剩余的挑战以及未来研究的可能方向。
更新日期:2020-04-06
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