Supercapacitors (SCs) have broad applications in wearable electronics (e.g., e-skin, robots). Recently, graphene-based supercapacitors (G-SCs) have attracted extensive attention for their excellent flexibility and electrochemical performance. Laser fabrication of G-SCs exhibits obvious superiority because of the simple procedures and integration compatibility with future electronics. Here, we comprehensively summarize the state-of-the-art advancements in laser-assisted preparation of G-SCs, including working mechanisms, fabrication procedures, and unique characteristics. In the working mechanism section, electric double-layer capacitors and pseudo-capacitors are introduced. The latest advancements in this field are comprehensively summarized, including laser reduction of graphene oxides, laser treatment of graphene prepared from chemical vapor deposition, and laser-induced graphene. In addition, the unique characteristics of laser-enabled G-SCs, such as structured graphene, graphene hybrids, and heteroatom doping graphene-related electrodes, are presented. Subsequently, laser-enabled miniaturized, stretchable, and integrated G-SCs are also discussed. It is anticipated that laser fabrication of G-SCs holds great promise for developing future energy storage devices.

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石墨烯基超级电容器的激光制造

超级电容器 (SC) 在可穿戴电子产品（例如电子皮肤、机器人）中具有广泛的应用。最近，基于石墨烯的超级电容器（G-SCs）因其优异的柔韧性和电化学性能而受到广泛关注。G-SCs 的激光制造具有明显的优势，因为它具有简单的程序和与未来电子产品的集成兼容性。在这里，我们全面总结了激光辅助制备 G-SCs 的最新进展，包括工作机制、制造程序和独特特性。在工作机理部分，介绍了双电层电容器和伪电容器。全面总结了该领域的最新进展，包括激光还原氧化石墨烯、化学气相沉积制备的石墨烯的激光处理和激光诱导石墨烯。此外，还介绍了激光启用的 G-SC 的独特特性，例如结构化石墨烯、石墨烯杂化和杂原子掺杂石墨烯相关电极。随后，还讨论了支持激光的小型化、可拉伸和集成 G-SC。预计 G-SC 的激光制造对于开发未来的储能设备具有广阔的前景。