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The role of associative ionization reactions in the memory effect of atmospheric pressure Townsend discharges in N 2 with a small O 2 addition
Journal of Physics D: Applied Physics ( IF 3.1 ) Pub Date : 2020-03-12 , DOI: 10.1088/1361-6463/ab7518
Xi Lin 1 , Clmence Tyl 1 , Nicolas Naud 1 , Nicolas Gherardi 1 , Nikolay A Popov 2, 3 , Simon Dap 1
Affiliation  

In this work, we investigate the role played by associative ionization reactions in the memory effect of atmospheric pressure Townsend dielectric barrier discharges working in N 2 with a small addition of O 2 . Systematic laser-induced fluorescence measurements are carried out in order to provide the absolute densities of N and O atoms and NO molecules for different oxygen concentrations. The use of these data in a dedicated model allows us, in particular, to estimate the rate of the reaction ##IMG## [http://ej.iop.org/images/0022-3727/53/20/205201/dab7518ieqn1.gif] {$\text{N(}^\text{2}\text{P)+O(}^\text{3}\text{P)}\rightarrow\text{NO}^\text{+}\text{+}\textit{e}$} suspected of playing a significant role. According to the obtained results, this reaction is found responsible for a significant enhancement in the production of seed electrons between two successive discharges at 25 ppm of O 2 , in good agreement with experimental obse...

中文翻译:

缔合电离反应在大气压下添加少量O 2的N 2中大气压Townsend放电的记忆效应中的作用

在这项工作中,我们研究了缔合电离反应在大气压下在少量添加O 2的N 2中工作的Townsend介电势垒放电的记忆效应中所起的作用。进行系统的激光诱导的荧光测量,以提供不同氧浓度下N和O原子以及NO分子的绝对密度。通过在专用模型中使用这些数据,我们尤其可以估算反应速率## IMG ## [http://ej.iop.org/images/0022-3727/53/20/205201/ dab7518ieqn1.gif] {$ \ text {N(} ^ \ text {2} \ text {P)+ O(} ^ \ text {3} \ text {P)} \ rightarrow \ text {NO} ^ \ text { +} \ text {+} \ textit {e} $}涉嫌扮演重要角色。根据获得的结果,
更新日期:2020-03-12
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