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Low amount of Au nanoparticles deposited ZnO nanorods heterojunction photocatalysts for efficient degradation of p -nitrophenol
Journal of Sol-Gel Science and Technology ( IF 2.5 ) Pub Date : 2020-02-12 , DOI: 10.1007/s10971-020-05249-4
Lei Bai , Jinxiang Mei

Abstract

By chemical precipitation of Au nanoparticles on the ZnO nanorods, the heterostructures were successfully obtained. The structures were investigated by several methods and it was revealed that with the increase of the Au precursor, the size of Au nanoparticles was increased and the interaction between Au nanoparticle and ZnO nanorod was also confirmed. The performance of the photodegradation of p-nitrophenol suggested that the activity was related with the amount of Au nanoparticles in Au/ZnO heterostructure to a great extent. It was suggested that by taking advantage of the one dimension ZnO nanorods with the effect of aspect ratio and surface defects as well as the local surface plasma resonance adsorption of Au nanoparticles, the heterostructures demonstrated an ideal activity under visible light for the disposal of low concentration of organic pollutants, suggesting a potential application in environmental remediation.

By taking advantage of one dimension ZnO nanorod with the effect of aspect ratio and surface defects as well as the local surface plasma resonance adsorption of Au nanoparticles, the Au nanoparticles/ZnO nanorods heterostructures were synthesized and demonstrated an ideal activity under visible light for the degradation of low concentration of organic pollutants.



中文翻译:

少量Au纳米颗粒沉积的ZnO纳米棒异质结光催化剂可有效降解对硝基苯酚

摘要

通过将金纳米颗粒化学沉淀在ZnO纳米棒上,成功获得了异质结构。通过几种方法对结构进行了研究,结果表明,随着Au前体的增加,Au纳米粒子的尺寸增加,并且证实了Au纳米粒子与ZnO纳米棒之间的相互作用。p的光降解性能-硝基苯酚表明其活性在很大程度上与Au / ZnO异质结构中Au纳米颗粒的数量有关。建议利用一维ZnO纳米棒的长径比和表面缺陷以及Au纳米颗粒的局部表面等离子体共振吸附效应,该异质结构在可见光下显示出理想的活性,可用于低浓度的处理。的有机污染物,表明其在环境修复中的潜在应用。

利用一维ZnO纳米棒的长径比和表面缺陷以及Au纳米颗粒的局部表面等离子体共振吸附的影响,合成了Au纳米颗粒/ ZnO纳米棒的异质结构,并在可见光下具有理想的降解活性。低浓度的有机污染物。

更新日期:2020-02-12
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