解决光催化二氧化碳还原的重现性
ChemCatChem
(
IF3.8
)
Pub Date : 2020-02-04, DOI: 10.1002/cctc.202000142
Maximilian Marx
1
,
Andrea Mele
2
,
Anke Spannenberg
1
,
Christoph Steinlechner
1
,
Henrik Junge
1
,
Philippe Schollhammer
2
,
Matthias Beller
1
Affiliation
Leibniz Institute for Catalysis at theUniversity of Rostock Albert-Einstein-Straße 29a Rostock 18059 Germany
UMR CNRS 6521 CEMCA Faculté des Sciences et TechniquesUniversity of Brest 6 Avenue Victor le Gorgeu Brest 29238 France
Addressing the Reproducibility of Photocatalytic Carbon Dioxide Reduction
The Front Cover shows mountain scenery on top of which the conversion of CO2 and water into CO, HCO2H and H2 mediated by light is depicted. Variable heights of the highlighted spots on the yellow mountain ridge (TON ridge) symbolize the fluctuant turnover numbers of a poorly reproducible catalytic reaction. In their Full Paper, M. Marx et al. outline problems with the reproducibility of photocatalytic transformations, specifically carbon dioxide reduction. Utilizing Fe hydrogenase mimics in combination with a Cu photosensitizer they highlight that complex equilibria and general problems associated with photocatalysis reaction set‐up can result in low reproducibility. Based on their results, suggestions are made on how to achieve higher reproducibility in such catalyst development. This main objective is also highlighted on the central signpost in the cover picture. More information can be found in the Full Paper by M. Marx et al..
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