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Synthesis of novel ternary g-C3N4/SiC/C-Dots photocatalysts and their visible-light-induced activities in removal of various contaminants
Journal of Photochemistry and Photobiology A: Chemistry ( IF 4.1 ) Pub Date : 2020-02-03 , DOI: 10.1016/j.jphotochem.2020.112431
Soheila Asadzadeh-Khaneghah , Aziz Habibi-Yangjeh , Mehdi Shahedi Asl , Zohre Ahmadi , Srabanti Ghosh

Different visible-light-driven nanocomposites were fabricated via combination of g-C3N4 (CN) with SiC and carbon dots (C-Dots) in the current research work. The features of photocatalysts were investigated by various analyses. The photocatalytic abilities were investigated by removal four aquatic pollutants. The outcomes demonstrated that the CN/SiC/C-Dots (0.25 mL) system has excellent photoability in the elimination of MB, fuchsine, RhB, and CR, which was about 26.9, 20.9, 24.4, and 15.2-folds premier than the single CN, respectively. The boosted photodegradation performance was related to the efficient separation of charges and high visible-light absorption, because of coupling CN with SiC and C-Dots. It was confirmed that the h+ and radical dotO2 plays essential roles in photocatalytic abilities. In our belief, this research work represents a novel method for the production of ternary metal-free nanocomposites based on CN, which could efficiently solve environmental crises.



中文翻译:

新型三元gC 3 N 4 / SiC / C-Dots光催化剂的合成及其可见光诱导的去除各种污染物的活性

在当前的研究工作中,通过将gC 3 N 4(CN)与SiC和碳点(C-Dots)相结合,制造了各种可见光驱动的纳米复合材料。通过各种分析研究了光催化剂的特征。通过去除四种水生污染物研究了光催化能力。结果表明,CN / SiC / C-Dots(0.25 mL)系统在消除MB,品红,RhB和CR方面具有出色的光敏性,比单分子主要高26.9、20.9、24.4和15.2倍。 CN,分别。由于CN与SiC和C-Dots的耦合,提高的光降解性能与电荷的有效分离和高可见光吸收率有关。证实了h +激进点O2 -起着催化能力的重要作用。我们相信,这项研究工作代表了一种新的生产基于CN的无金属三元纳米复合材料的方法,该方法可以有效解决环境危机。

更新日期:2020-02-03
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