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Defect Engineering on Electrode Materials for Rechargeable Batteries.
Advanced Materials ( IF 27.4 ) Pub Date : 2020-01-13 , DOI: 10.1002/adma.201905923
Yiqiong Zhang 1, 2 , Li Tao 1 , Chao Xie 1 , Dongdong Wang 1 , Yuqin Zou 1 , Ru Chen 1 , Yanyong Wang 1 , Chuankun Jia 2 , Shuangyin Wang 1
Affiliation  

The reasonable design of electrode materials for rechargeable batteries plays an important role in promoting the development of renewable energy technology. With the in-depth understanding of the mechanisms underlying electrode reactions and the rapid development of advanced technology, the performance of batteries has significantly been optimized through the introduction of defect engineering on electrode materials. A large number of coordination unsaturated sites can be exposed by defect construction in electrode materials, which play a crucial role in electrochemical reactions. Herein, recent advances regarding defect engineering in electrode materials for rechargeable batteries are systematically summarized, with a special focus on the application of metal-ion batteries, lithium-sulfur batteries, and metal-air batteries. The defects can not only effectively promote ion diffusion and charge transfer but also provide more storage/adsorption/active sites for guest ions and intermediate species, thus improving the performance of batteries. Moreover, the existing challenges and future development prospects are forecast, and the electrode materials are further optimized through defect engineering to promote the development of the battery industry.

中文翻译:

可充电电池电极材料的缺陷工程。

充电电池电极材料的合理设计在促进可再生能源技术的发展中起着重要作用。随着对电极反应机理的深入理解和先进技术的迅速发展,通过在电极材料上引入缺陷工程,电池的性能得到了极大的优化。电极材料中的缺陷结构可暴露出大量配位不饱和位点,这在电化学反应中起着至关重要的作用。在此,系统地总结了关于可再充电电池的电极材料中的缺陷工程的最新进展,特别着重于金属离子电池,锂硫电池和金属空气电池的应用。这些缺陷不仅可以有效地促进离子扩散和电荷转移,还可以为客体离子和中间物种提供更多的存储/吸附/活性位点,从而提高电池的性能。此外,对存在的挑战和未来的发展前景进行了预测,并通过缺陷工程进一步优化了电极材料,以促进电池工业的发展。
更新日期:2020-02-18
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