Research on Chemical Intermediates ( IF 2.8 ) Pub Date : 2020-01-13 , DOI: 10.1007/s11164-019-04070-1 Venkata Rao Madduluri , Raju Narsinga , Dosa Mallesh , P. Mahesh Kumar , Shankar Barapati , Sreedhar Bojja , Kamaraju Seetha Rama Rao
A series of lanthanum oxide (La2O3—2–14 wt%)-encapsulated Co3O4/MgO catalysts and bare Co/MgO solid oxides were prepared by wetness impregnation method. Among all catalysts, La2O3-promoted Co3O4/MgO (CM) was found to be remarkable in terms of superior promotional effect of La oxide species. Therefore, La2O3-incorporated Co3O4/MgO (LCM) catalysts afforded unusual catalytic activity efficiency with respect to high EB conversion and styrene selectivity due to the synergistic effect of Co–La species. By contrast, bare Co3O4/MgO solid oxide (CM) catalyst afforded low EB conversion with mild catalytic activity due to the absence of promotional role of La oxide.
中文翻译:
Co 3 O 4 / MgO催化剂上Co 3 O 4浸渍的La 2 O 3 / MgO在乙苯的氧化脱氢中的催化性能提高
采用湿法浸渍法制备了一系列包埋氧化镧(La 2 O 3 -2-14 wt%)的Co 3 O 4 / MgO催化剂和裸露的Co / MgO固体氧化物。在所有催化剂中,发现La 2 O 3促进的Co 3 O 4 / MgO(CM)就La氧化物种类的优异促进效果而言是显着的。因此,由于Co-La的协同作用,结合La 2 O 3的Co 3 O 4 / MgO(LCM)催化剂在高EB转化率和苯乙烯选择性方面提供了非同寻常的催化活性效率。相比之下,裸Co3 O 4 / MgO固体氧化物(CM)催化剂提供了低的EB转化率,并且由于没有La氧化物的促进作用而具有中等的催化活性。