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The Rise of Textured Perovskite Morphology: Revolutionizing the Pathway toward High‐Performance Optoelectronic Devices
Advanced Energy Materials ( IF 24.4 ) Pub Date : 2020-01-10 , DOI: 10.1002/aenm.201902256
Jun‐Xing Zhong 1 , Wu‐Qiang Wu 1, 2 , Jin‐Feng Liao 1 , Wenhuai Feng 1 , Yong Jiang 1 , Lianzhou Wang 2 , Dai‐Bin Kuang 1
Affiliation  

Halide perovskite materials have achieved overwhelming success in various optoelectronic applications, especially perovskite solar cells and perovskite‐based light‐emitting diodes (P‐LEDs), owing to their outstanding optical and electric properties. It is widely believed that flat and mirror‐like perovskite films are imperative for achieving high device performance, while the potential of other perovskite morphologies, such as the emerging textured perovskite, is overlooked, which leaves plenty of room for further breakthroughs. Compared to flat and mirror‐like perovskites, textured perovskites with unique structures, e.g., coral‐like, maze‐like, column‐like or quasi‐core@shell assemblies, are more efficient at light harvesting and charge extraction, thus revolutionizing the pathways toward ultrahigh performance in perovskite‐based optoelectronic devices. Employing a textured perovskite morphology, the record of external quantum efficiency for P‐LEDs is demonstrated as 21.6%. In this research news, recent progress in the utilization of textured perovskite is summarized, with the emphasis on the preparation strategies and prominent optoelectronic properties. The impact of the textured morphology on light harvesting, carrier dynamic management, and device performance is highlighted. Finally, the challenges and great potential of employing these innovative morphologies in fabricating more efficient optoelectronic devices, or creating a new energy harvesting and conversion regime are also provided.

中文翻译:

钙钛矿纹理形态的兴起:革新了高性能光电器件的发展途径

卤化物钙钛矿材料由于其出色的光学和电学性能,在各种光电应用中取得了压倒性的成功,尤其是钙钛矿太阳能电池和钙钛矿基发光二极管(P-LED)。普遍认为,平面和镜面钙钛矿膜对于实现高设备性能必不可少,而其他钙钛矿形态的潜力(例如新兴的纹理钙钛矿)却被忽略了,这为进一步的突破留出了很大的空间。与平面和镜面钙钛矿相比,具有独特结构的纹理钙钛矿,例如珊瑚状,迷宫状,圆柱状或准核@壳装配体,在光收集和电荷提取方面效率更高,因此,彻底改变了基于钙钛矿的光电设备实现超高性能的途径。利用纹理化的钙钛矿形态,P-LED的外部量子效率记录显示为21.6%。在此研究新闻中,总结了带纹理的钙钛矿利用的最新进展,重点是制备策略和突出的光电性能。强调了纹理形态对光收集,载流子动态管理和设备性能的影响。最后,还提供了使用这些创新形态来制造更高效的光电器件或创建新的能量收集和转换方案的挑战和巨大潜力。P‐LED的外部量子效率记录显示为21.6%。在此研究新闻中,总结了带纹理的钙钛矿利用的最新进展,重点是制备策略和突出的光电性能。强调了纹理形态对光收集,载流子动态管理和设备性能的影响。最后,还提供了使用这些创新形态来制造更高效的光电器件或创建新的能量收集和转换方案的挑战和巨大潜力。P‐LED的外部量子效率记录显示为21.6%。在此研究新闻中,总结了带纹理的钙钛矿利用的最新进展,重点是制备策略和突出的光电性能。强调了纹理形态对光收集,载流子动态管理和设备性能的影响。最后,还提供了使用这些创新形态来制造更高效的光电器件或创建新的能量收集和转换方案的挑战和巨大潜力。强调了纹理形态对光收集,载流子动态管理和设备性能的影响。最后,还提供了使用这些创新形态来制造更高效的光电器件或创建新的能量收集和转换方案的挑战和巨大潜力。强调了纹理形态对光收集,载流子动态管理和设备性能的影响。最后,还提供了使用这些创新形态来制造更高效的光电器件或创建新的能量收集和转换方案的挑战和巨大潜力。
更新日期:2020-02-18
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