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Metal–Organic Framework-Based Materials for Energy Conversion and Storage
ACS Energy Letters ( IF 19.3 ) Pub Date : 2020-01-23 , DOI: 10.1021/acsenergylett.9b02625
Tianjie Qiu 1, 2 , Zibin Liang 1, 2 , Wenhan Guo 1, 2 , Hassina Tabassum 1, 2 , Song Gao 1, 2 , Ruqiang Zou 1, 2
Affiliation  

Metal–organic frameworks (MOFs) have emerged as desirable cross-functional platforms for electrochemical and photochemical energy conversion and storage (ECS) systems owing to their highly ordered and tunable compositions and structures. In this Review, we present engineering principles promoting the electro-/photochemical performance of MOF-based materials for ECS by component design and nanostructuring. Through the discussion of the engineering strategies of pristine MOFs, MOF composites, and their derivatives for ECS, the superiority and composition–structure–activity relationships of the engineered MOF-based materials with advanced components and nanostructures will be clarified. Finally, we provide a concluding discussion on the challenges and direction of future development in this emerging area of MOF-based materials for ECS.

中文翻译:

基于金属有机框架的材料,用于能量转换和存储

金属有机框架(MOF)由于其高度有序且可调节的组成和结构,已成为电化学和光化学能转换和存储(ECS)系统的理想跨功能平台。在这篇评论中,我们介绍了通过组件设计和纳米结构促进基于MOF的材料在ECS中的电/光化学性能的工程原理。通过讨论原始MOF,MOF复合材料及其衍生物用于ECS的工程策略,将阐明具有先进组件和纳米结构的MOF基工程材料的优越性以及组成,结构与活性之间的关系。最后,我们就基于MOF的ECS材料这一新兴领域中的挑战和未来发展方向提供了总结性讨论。
更新日期:2020-01-23
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