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Two-dimensional metal–organic frameworks and their derivatives for electrochemical energy storage and electrocatalysis
Nanoscale Advances ( IF 4.6 ) Pub Date : 2020/01/06 , DOI: 10.1039/c9na00719a Kuangmin Zhao 1 , Weiwei Zhu 1 , Suqin Liu 1 , Xianli Wei 1 , Guanying Ye 1 , Yuke Su 1 , Zhen He 1
Nanoscale Advances ( IF 4.6 ) Pub Date : 2020/01/06 , DOI: 10.1039/c9na00719a Kuangmin Zhao 1 , Weiwei Zhu 1 , Suqin Liu 1 , Xianli Wei 1 , Guanying Ye 1 , Yuke Su 1 , Zhen He 1
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Two-dimensional (2D) metal–organic frameworks (MOFs) and their derivatives with excellent dimension-related properties, e.g. high surface areas, abundantly accessible metal nodes, and tailorable structures, have attracted intensive attention as energy storage materials and electrocatalysts. A major challenge on the road toward the commercialization of 2D MOFs and their derivatives is to achieve the facile and controllable synthesis of 2D MOFs with high quality and at low cost. Significant developments have been made in the synthesis and applications of 2D MOFs and their derivatives in recent years. In this review, we first discuss the state-of-the-art synthetic strategies (including both top-down and bottom-up approaches) for 2D MOFs. Subsequently, we review the most recent application progress of 2D MOFs and their derivatives in the fields of electrochemical energy storage (e.g., batteries and supercapacitors) and electrocatalysis (of classical reactions such as the HER, OER, ORR, and CO2RR). Finally, the challenges and promising strategies for the synthesis and applications of 2D MOFs and their derivatives are addressed for future development.
中文翻译：
用于电化学储能和电催化的二维金属有机框架及其衍生物
二维（2D）金属有机框架（MOF）及其衍生物具有优异的尺寸相关特性，例如高表面积、丰富的金属节点和可定制的结构，作为储能材料和电催化剂引起了人们的广泛关注。二维MOFs及其衍生物商业化道路上的一个主要挑战是实现高质量、低成本的简便可控合成2D MOFs。近年来，二维MOFs及其衍生物的合成和应用取得了重大进展。在这篇综述中，我们首先讨论了 2D MOF 的最先进的合成策略（包括自上而下和自下而上的方法）。随后，我们回顾了2D MOFs及其衍生物在电化学储能（如电池和超级电容器）和电催化（HER、OER、ORR和CO 2 RR等经典反应）领域的最新应用进展。最后，讨论了二维 MOF 及其衍生物的合成和应用面临的挑战和有前景的策略，以供未来发展。
更新日期：2020-02-19
中文翻译：
用于电化学储能和电催化的二维金属有机框架及其衍生物
二维（2D）金属有机框架（MOF）及其衍生物具有优异的尺寸相关特性，例如高表面积、丰富的金属节点和可定制的结构，作为储能材料和电催化剂引起了人们的广泛关注。二维MOFs及其衍生物商业化道路上的一个主要挑战是实现高质量、低成本的简便可控合成2D MOFs。近年来，二维MOFs及其衍生物的合成和应用取得了重大进展。在这篇综述中，我们首先讨论了 2D MOF 的最先进的合成策略（包括自上而下和自下而上的方法）。随后，我们回顾了2D MOFs及其衍生物在电化学储能（如电池和超级电容器）和电催化（HER、OER、ORR和CO 2 RR等经典反应）领域的最新应用进展。最后，讨论了二维 MOF 及其衍生物的合成和应用面临的挑战和有前景的策略，以供未来发展。
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