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Construction of nanoporous gold/g-C3N4 heterostructure for electrochemical supercapacitor
Electrochimica Acta ( IF 5.5 ) Pub Date : 2018-10-16 , DOI: 10.1016/j.electacta.2018.10.106
A.Y. Chen , T.T. Zhang , Y.J. Qiu , D. Wang , P. Wang , H.J. Li , Y. Li , J.H. Yang , X.Y. Wang , X.F. Xie

Hybrids with two-dimensional and three-dimensional nanostructures have attracted great interest in the construction of supercapacitor electrodes due to their unique structural features. Graphitic carbon nitride (g-C3N4) nanosheets are deposited on the surface of a nanoporous gold (NPG) film via an electrochemical method to form a hybrid electrode of NPG/g-C3N4 with an ultra-thin, ultra-light and good flexible characteristics. The electrochemical tests show that the hybrid electrode exhibits a good supercapacitive performance, such as an admirable specific capacitance (440 F g−1 at 2 A g−1) in 0.5 M Na2SO4 solution and a favorable cycling durability (maintaining 98% capacity after 10000 cycles). More interesting, the NPG/g-C3N4 electrode displays a striking enhancement of supercapacitive performance with the increase of bending angle. This superior property can be attributed to the unique nanosheets on nanoporous structure by a strong interfacial effect between the defected Au atoms of NPG and g-C3N4.



中文翻译:

电化学超级电容器纳米多孔金/ gC 3 N 4异质结构的构建

具有二维和三维纳米结构的混合体因其独特的结构特征而引起了超级电容器电极的极大兴趣。通过电化学方法将石墨化的氮化碳(gC 3 N 4)纳米片沉积在纳米多孔金(NPG)膜的表面上,以形成具有超薄,超轻且优质的NPG / gC 3 N 4混合电极。灵活的特点。电化学测试表明,混合电极显示出良好的性能超级电容,诸如极佳的比电容(440 F G -1在2A克-1在0.5M的Na)2 SO 4解决方案和良好的循环耐久性(10000次循环后仍保持98%的容量)。更有趣的是,NPG / gC 3 N 4电极随着弯曲角的增加而显示出超电容性能的显着增强。NPG的缺陷Au原子和gC 3 N 4之间的强界面作用可归因于纳米多孔结构上独特的纳米片。

更新日期:2018-10-16
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