MOFs‐Based Heterogeneous Catalysts: New Opportunities for Energy‐Related CO2 Conversion,Advanced Energy Materials

当前位置： X-MOL 学术 › Adv. Energy Mater. › 论文详情

Our official English website, www.x-mol.net, welcomes your feedback! (Note: you will need to create a separate account there.)

MOFs‐Based Heterogeneous Catalysts: New Opportunities for Energy‐Related CO2 Conversion
Advanced Energy Materials ( IF 24.4 ) Pub Date : 2018-10-14 , DOI: 10.1002/aenm.201801587
Zhendong Lei _{1,

2} , Yuancheng Xue ₃ , Wenqian Chen ₃ , Wenhui Qiu _{4,

5} , Yong Zhang ₂ , Satoshi Horike ₆ , Liang Tang ₁

Affiliation

Metal–organic frameworks (MOFs) with high surface area and tunable chemical structures have attracted tremendous attention. Recently, the utilization of solar energy for CO₂ conversion to produce valuable chemicals or fuels has become extremely appealing. The interior of MOFs can be designed to have defects, heteroatoms and embedded nanoscale metal catalysts for the development of CO₂ conversion. In this review, the recent development of MOFs‐based catalysts for CO₂ conversion reactions, including photocatalysis and electrocatalysis are summarized. In particular, the preparation and mechanism of CO₂ conversion‐based MOFs are discussed. The examples are expected to provide deeper understanding in preparing highly active and stable MOFs‐based CO₂ conversion materials.

中文翻译：

基于MOF的多相催化剂：与能源相关的CO2转化的新机会

具有高表面积和可调节化学结构的金属有机框架（MOF）引起了极大的关注。近来，利用太阳能进行CO ₂转化以生产有价值的化学物质或燃料已变得极具吸引力。MOF的内部可以设计成具有缺陷，杂原子和嵌入式纳米级金属催化剂，以促进CO ₂转化。在这篇综述中，总结了基于MOFs的催化剂在CO ₂转化反应中的最新进展，包括光催化和电催化。特别是CO ₂的制备及其机理讨论了基于转换的MOF。这些示例有望在制备高活性和稳定的基于MOF的CO ₂转化材料时提供更深刻的理解。

更新日期：2018-10-14

点击分享查看原文

点击收藏

阅读更多本刊最新论文本刊介绍/投稿指南11