当前位置: X-MOL 学术J. Nucl. Mater. › 论文详情
Our official English website, www.x-mol.net, welcomes your feedback! (Note: you will need to create a separate account there.)
In-situ TEM study of the ion irradiation behavior of U3Si2 and U3Si5
Journal of Nuclear Materials ( IF 3.1 ) Pub Date : 2018-08-31 , DOI: 10.1016/j.jnucmat.2018.08.058
Tiankai Yao , Bowen Gong , Lingfeng He , Yinbin Miao , Jason M. Harp , Michael Tonks , Jie Lian

U3Si2 and U3Si5 are two important uranium silicide phases currently under extensive investigation as potential fuel forms or components for light water reactors (LWRs) to enhance accident tolerance. In this paper, their irradiation behaviors are studied by ion beam irradiations with various ion mass and energies, and their microstructure evolution is investigated by in-situ transmission electron microscopy (TEM). U3Si2 can easily be amorphized by ion beam irradiations (by 1 MeV Ar2+ or Kr2+) at room temperature with the critical amorphization dose less than 1 dpa. The critical amorphization temperatures of U3Si2 irradiated by 1 MeV Kr2+ and 1 MeV Ar2+ ion are determined as 580 ± 10 K and 540 ± 5 K, respectively. In contrast, U3Si5 remains crystalline up to 8 dpa at room temperature and is stable against ion irradiation-induced amorphization up to ∼50 dpa by either 1 MeV Kr2+ or 150 KeV Kr+ at 623 K. These results provide valuable experimental data to guide future irradiation experiments, support the relevant post irradiation examination, and serve as the experimental basis for the validation of advanced fuel performance models.



中文翻译:

U 3 Si 2和U 3 Si 5的离子辐照行为的原位TEM研究

U 3 Si 2和U 3 Si 5是两个重要的硅化铀重要相,目前正作为轻水反应堆(LWR)的潜在燃料形式或组分,以提高事故承受能力,正在对其进行广泛研究。在本文中,通过各种离子质量和能量的离子束辐照研究了它们的辐照行为,并通过原位透射电子显微镜(TEM)研究了它们的微观结构演变。U 3 Si 2可以通过离子束辐照(通过1 MeV Ar 2+或Kr 2+)在室温下且临界非晶化剂量小于1 dpa。1 MeV Kr 2+和1 MeV Ar 2+离子辐照的U 3 Si 2的临界非晶化温度分别确定为580±10 K和540±5K。相比之下,U 3 Si 5在室温下保持高达8 dpa的结晶状态,并且对于1 MeV Kr 2+或150 KeV Kr +的离子辐照引起的高达50 dpa的非晶化具有稳定作用。 在623 K时。这些结果提供了宝贵的实验数据,可指导未来的辐照实验,支持相关的辐照后检查,并为验证先进燃料性能模型提供实验基础。

更新日期:2018-08-31
down
wechat
bug