The radical acylarylation of N-arylacrylamides with aliphatic aldehydes using the photolysis of hypervalent iodine(iii) reagents†,Organic & Biomolecular Chemistry

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The radical acylarylation of N-arylacrylamides with aliphatic aldehydes using the photolysis of hypervalent iodine(iii) reagents†
Organic & Biomolecular Chemistry ( IF 2.9 ) Pub Date : 2018-07-14 00:00:00 , DOI: 10.1039/c8ob01420e
Ryu Sakamoto _{1,

2,

3,

4,

5} , Naomichi Hirama _{1,

2,

3,

4,

5} , Keiji Maruoka _{1,

2,

3,

4,

5}

Affiliation

This article describes a variety of 3,3-disubstituted 2-oxindoles that bear carbonyl groups, which are efficiently obtained from a radical reaction between N-arylacrylamides and aliphatic aldehydes. The reaction is initiated by the photolysis of hypervalent iodine(III) reagents and proceeds smoothly under mild, metal-free conditions.

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