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Synthesis of solution processed [email protected]2S3 hybrid film coated linen fabric as a free-standing textile structured photo catalyst
Applied Catalysis A: General ( IF 4.7 ) Pub Date : 2018-06-10 , DOI: 10.1016/j.apcata.2018.06.015
Anam Ali Memon , Alvira Ayoub Arbab , Supriya A. Patil , Naveed Mengal , Kyung Chul Sun , Iftikhar Ali Sahito , Sung Hoon Jeong , Hak Sung Kim

A unique metallic carbon hybrid film, synthesized with synchronized distribution of bismuth sulfide (Bi2S3) and exfoliated multiwall carbon nanotubes (MWCNTs), has been proposed for use as freestanding textile electrodes in photo catalysts. The defect-rich morphology of Bi2S3 nanowire decorated MWCNT hybrid enhances the photocatalytic activity, electronic properties, cyclic stability, and electron pathways. The proposed [email protected]2S3-hybrid linen fabric electrode demonstrated a defect-rich morphology synchronized with high electrical conductivity. These properties greatly enhanced the photocatalytic activity and electron transfer. The high photocatalytic activity is attributed to the synergistic effect of the high electron affinity of MWCNTs and the structural distortion caused by Bi2S3 nanowires. Degradation of methylene blue dye was accelerated owing to the elevated activity of Bi2S3 nanowires, which provides fast absorption of contaminants and reduction of oxidative species. Our proposed system of metallic carbon freestanding textile electrode opens the broad applications of textile-based photochemical devices.



中文翻译:

溶液处理的[受电子邮件保护] 2 S 3杂化膜涂层亚麻织物的合成,作为自立式纺织结构光催化剂

已经提出了一种独特的金属碳杂化膜,该膜由硫化铋(Bi 2 S 3)和剥离的多壁碳纳米管(MWCNTs)的同步分布合成而成,可用作光催化剂中的独立式纺织电极。Bi 2 S 3纳米线修饰的MWCNT杂化物的富缺陷形态增强了光催化活性,电子性能,循环稳定性和电子途径。建议[电子邮件保护的] 2 S 3-混合亚麻织物电极表现出与高电导率同步的富缺陷形态。这些性质大大增强了光催化活性和电子转移。高的光催化活性归因于MWCNT的高电子亲和力和Bi 2 S 3纳米线引起的结构变形的协同效应。由于Bi 2 S 3纳米线的活性提高,亚甲基蓝染料的降解得以加速,这可以快速吸收污染物并减少氧化性物质。我们建议的金属碳独立式纺织品电极系统打开了基于纺织品的光化学装置的广泛应用。

更新日期:2018-06-10
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