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Nano-designed semiconductors for electro- and photoelectro-catalytic conversion of carbon dioxide
Chemical Society Reviews ( IF 40.4 ) Pub Date : 2018-05-25 00:00:00 , DOI: 10.1039/c8cs00016f
Lei Zhang 1, 2, 3, 4, 5 , Zhi-Jian Zhao 1, 2, 3, 4, 5 , Tuo Wang 1, 2, 3, 4, 5 , Jinlong Gong 1, 2, 3, 4, 5
Affiliation  

Development of novel catalysts with high efficiency for CO2 conversion is of great research interest, because of the climate hazards caused by the gradual increase in CO2 concentration. Among various types of catalysts, semiconductors have been widely used as effective candidates for both electro- and photoelectro-CO2 conversion. Very recently, with the emerging nanotechnology and advanced characterization techniques, tremendous achievements have been made in highly efficient and clean CO2 conversion based on semiconductor catalysts. This review gives a systematic overview of this field, including the rational design of semiconductor catalysts for electro- and photoelectro-chemical CO2 conversion. Recent advances in the development of mechanism understandings on reaction pathways of CO2 and the feasibility for industrial production are discussed. Furthermore, the challenges and future perspectives of electro- and photoelectro-catalytic CO2 conversion are outlined.

中文翻译:

纳米设计的半导体,用于二氧化碳的电催化和光电催化转化

由于由CO 2浓度的逐渐增加引起的气候危害,开发具有高效率的用于CO 2转化的新型催化剂具有极大的研究兴趣。在各种类型的催化剂中,半导体已被广泛用作电和光-CO 2转化的有效候选物。最近,随着新兴的纳米技术和先进的表征技术,在基于半导体催化剂的高效,清洁的CO 2转化中取得了巨大的成就。这篇综述对这一领域进行了系统的概述,包括合理设计用于电化学和光电化学CO 2的半导体催化剂转换。讨论了对CO 2反应途径的机理理解的最新进展以及工业生产的可行性。此外,概述了电催化和光电催化CO 2转化的挑战和未来前景。
更新日期:2018-05-25
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