Nano-designed semiconductors for electro- and photoelectro-catalytic conversion of carbon dioxide,Chemical Society Reviews

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Nano-designed semiconductors for electro- and photoelectro-catalytic conversion of carbon dioxide
Chemical Society Reviews ( IF 40.4 ) Pub Date : 2018-05-25 00:00:00 , DOI: 10.1039/c8cs00016f
Lei Zhang _{1,

2,

3,

4,

5} , Zhi-Jian Zhao _{1,

2,

3,

4,

5} , Tuo Wang _{1,

2,

3,

4,

5} , Jinlong Gong _{1,

2,

3,

4,

5}

Affiliation

Development of novel catalysts with high efficiency for CO₂ conversion is of great research interest, because of the climate hazards caused by the gradual increase in CO₂ concentration. Among various types of catalysts, semiconductors have been widely used as effective candidates for both electro- and photoelectro-CO₂ conversion. Very recently, with the emerging nanotechnology and advanced characterization techniques, tremendous achievements have been made in highly efficient and clean CO₂ conversion based on semiconductor catalysts. This review gives a systematic overview of this field, including the rational design of semiconductor catalysts for electro- and photoelectro-chemical CO₂ conversion. Recent advances in the development of mechanism understandings on reaction pathways of CO₂ and the feasibility for industrial production are discussed. Furthermore, the challenges and future perspectives of electro- and photoelectro-catalytic CO₂ conversion are outlined.

中文翻译：

纳米设计的半导体，用于二氧化碳的电催化和光电催化转化

由于由CO ₂浓度的逐渐增加引起的气候危害，开发具有高效率的用于CO ₂转化的新型催化剂具有极大的研究兴趣。在各种类型的催化剂中，半导体已被广泛用作电和光-CO ₂转化的有效候选物。最近，随着新兴的纳米技术和先进的表征技术，在基于半导体催化剂的高效，清洁的CO ₂转化中取得了巨大的成就。这篇综述对这一领域进行了系统的概述，包括合理设计用于电化学和光电化学CO ₂的半导体催化剂转换。讨论了对CO ₂反应途径的机理理解的最新进展以及工业生产的可行性。此外，概述了电催化和光电催化CO ₂转化的挑战和未来前景。

更新日期：2018-05-25

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