Recent progress in two-dimensional polymers for energy storage and conversion: design, synthesis, and applications,Journal of Materials Chemistry A

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Recent progress in two-dimensional polymers for energy storage and conversion: design, synthesis, and applications
Journal of Materials Chemistry A ( IF 10.7 ) Pub Date : 2018-05-09 00:00:00 , DOI: 10.1039/c8ta02820f
Peitao Xiao _{1,

2,

3,

4,

5} , Yuxi Xu _{1,

2,

3,

4,

5}

Affiliation

The increasing concerns about environmental issues caused by fossil fuels, and the demand for renewable energy have trigged extensive research into efficient energy storage and conversion systems. Owning to their unique properties of a high specific area, well-defined pore size, and tunable molecular structure, 2D metal–organic frameworks (MOFs) and covalent–organic frameworks (COFs), as two typical classes of 2D porous polymers, have been considered as intriguing materials for energy storage and conversion. This review provides a comprehensive overview of the up-to-date synthesis strategies of 2D MOFs and COFs, and their further applications. We mainly focus on the top-down and bottom-up synthesis methods, and applications in supercapacitors, lithium-ion batteries, batteries beyond lithium-ion batteries (lithium–sulfur batteries, and sodium-ion batteries), and electrocatalysts for CO₂ reduction, oxygen evolution, oxygen reduction, and hydrogen evolution.

中文翻译：

用于能量存储和转换的二维聚合物的最新进展：设计，合成和应用

对由化石燃料引起的环境问题以及对可再生能源的需求的日益关注，促使人们对有效的能量存储和转换系统进行了广泛的研究。由于具有高比表面积，定义明确的孔径和可调节的分子结构的独特特性，二维金属-有机骨架（MOF）和共价-有机骨架（COF）作为二维多孔聚合物的两大典型类别，已经得到了广泛应用。被认为是用于能量存储和转换的有趣材料。这篇综述全面概述了2D MOF和COF的最新合成策略，以及它们的进一步应用。我们主要关注自上而下和自下而上的合成方法，以及在超级电容器，锂离子电池，锂离子电池以外的电池（锂硫电池，₂还原，氧气析出，氧气还原和析氢。

更新日期：2018-05-09

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