Perovskite Solar Absorbers: Materials by Design,Small Methods

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Perovskite Solar Absorbers: Materials by Design
Small Methods ( IF 10.7 ) Pub Date : 2018-03-24 , DOI: 10.1002/smtd.201700316
Qiaoling Xu ₁ , Dongwen Yang ₁ , Jian Lv ₁ , Yi-Yang Sun ₂ , Lijun Zhang _{1,

3}

Affiliation

Solar‐cell materials with a tetrahedral diamond structure and its derived structures (i.e., zinc blende and chalcopyrite) are the most successful family of materials, with power conversion efficiencies exceeding 20%. Recent breakthroughs based on lead halide perovskites have inspired intensive research on low‐cost photovoltaics beyond diamond‐structured materials. While research has focused on addressing the key challenges faced by lead halide perovskites, that is, the stability and toxicity issues, it is of greater interest to develop perovskites into a new family of solar‐cell materials. Here, the recent efforts toward this goal are reviewed. The focus is on computational materials design, including single, double, 2D, and nonhalide perovskites and perovskite‐like materials. Meanwhile, related experiments are also reviewed with a hope that such this will help identify potential issues as well as enlightening ideas to achieve further computation‐driven materials discovery.

中文翻译：

钙钛矿型太阳能吸收剂：按设计的材料

具有四面体金刚石结构及其衍生结构的太阳能电池材料（即锌共混物和黄铜矿）是最成功的材料家族，其功率转换效率超过20％。基于卤化钙钛矿的最新突破启发了人们对除金刚石结构材料之外的低成本光伏电池的深入研究。虽然研究的重点是解决卤化钙钛矿含铅面临的主要挑战，即稳定性和毒性问题，但将钙钛矿开发成太阳能电池材料的新系列，将引起更大的兴趣。在此，回顾了为实现该目标所做的最新努力。重点是计算材料设计，包括单，双，二维和非卤化物钙钛矿和类钙钛矿材料。同时，

更新日期：2018-03-24

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