Mechanical Properties in Metal–Organic Frameworks: Emerging Opportunities and Challenges for Device Functionality and Technological Applications,Advanced Materials

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Mechanical Properties in Metal–Organic Frameworks: Emerging Opportunities and Challenges for Device Functionality and Technological Applications
Advanced Materials ( IF 27.4 ) Pub Date : 2017-11-17 , DOI: 10.1002/adma.201704124
Nicholas C. Burtch ₁ , Jurn Heinen ₂ , Thomas D. Bennett ₃ , David Dubbeldam ₂ , Mark D. Allendorf ₁

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Some of the most remarkable recent developments in metal–organic framework (MOF) performance properties can only be rationalized by the mechanical properties endowed by their hybrid inorganic–organic nanoporous structures. While these characteristics create intriguing application prospects, the same attributes also present challenges that will need to be overcome to enable the integration of MOFs with technologies where these promising traits can be exploited. In this review, emerging opportunities and challenges are identified for MOF‐enabled device functionality and technological applications that arise from their fascinating mechanical properties. This is discussed not only in the context of their more well‐studied gas storage and separation applications, but also for instances where MOFs serve as components of functional nanodevices. Recent advances in understanding MOF mechanical structure–property relationships due to attributes such as defects and interpenetration are highlighted, and open questions related to state‐of‐the‐art computational approaches for quantifying their mechanical properties are critically discussed.

中文翻译：

金属有机框架中的机械性能：设备功能和技术应用的新兴机遇与挑战

金属-有机骨架（MOF）性能特性的一些最近最显着的发展只能通过它们的无机-有机纳米多孔混合结构所赋予的机械性能来合理化。尽管这些特性创造了诱人的应用前景，但相同的属性也带来了挑战，必须克服这些挑战才能使MOF与可以利用这些有希望的特性的技术集成。在本文中，由于其出色的机械性能，为启用MOF的设备功能和技术应用确定了新的机遇和挑战。这不仅是在对其气体存储和分离技术有更深入研究的背景下讨论的，而且在MOF充当功能纳米设备的组件的情况下也进行了讨论。

更新日期：2017-11-17

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