Synthesis of 2D Metal Chalcogenide Thin Films through the Process Involving Solution‐Phase Deposition,Advanced Materials

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Synthesis of 2D Metal Chalcogenide Thin Films through the Process Involving Solution‐Phase Deposition
Advanced Materials ( IF 27.4 ) Pub Date : 2018-04-24 , DOI: 10.1002/adma.201707577
Anupam Giri ₁ , Gyeongbae Park ₁ , Heeseung Yang ₂ , Monalisa Pal ₁ , Junghyeok Kwak ₁ , Unyong Jeong ₁

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2D metal chalcogenide thin films have recently attracted considerable attention owing to their unique physicochemical properties and great potential in a variety of applications. Synthesis of large‐area 2D metal chalcogenide thin films in controllable ways remains a key challenge in this research field. Recently, the solution‐based synthesis of 2D metal chalcogenide thin films has emerged as an alternative approach to vacuum‐based synthesis because it is relatively simple and easy to scale up for high‐throughput production. In addition, solution‐based thin films open new opportunities that cannot be achieved from vacuum‐based thin films. Here, a comprehensive summary regarding the basic structures and properties of different types of 2D metal chalcogenides, the mechanistic details of the chemical reactions in the synthesis of the metal chalcogenide thin films, recent successes in the synthesis by different reaction approaches, and the applications and potential uses is provided. In the last perspective section, the technical challenges to be overcome and the future research directions in the solution‐based synthesis of 2D metal chalcogenides are discussed.

中文翻译：

固溶相沉积法合成二维金属硫属化物薄膜

二维金属硫族化物薄膜由于其独特的理化性质和在各种应用中的巨大潜力，最近引起了广泛的关注。以可控方式合成大面积二维金属硫属化物薄膜仍然是该研究领域的关键挑战。最近，基于溶液的2D金属硫族化物薄膜合成已经成为基于真空的合成的替代方法，因为它相对简单且易于扩大规模以用于高通量生产。此外，基于解决方案的薄膜还开辟了真空基薄膜无法实现的新机遇。这里是有关不同类型的2D金属硫属元素化物的基本结构和性质的综合摘要，提供了金属硫属化物薄膜的合成中化学反应的机理细节，通过不同反应方法合成的最新成功及其应用和潜在用途。在最后一个视角部分中，讨论了要解决的技术难题以及在基于溶液的二维金属硫属化物合成中的未来研究方向。

更新日期：2018-04-24

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