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Absorption of SO2 with calcium-based solution in a rotating packed bed
Separation and Purification Technology ( IF 8.6 ) Pub Date : 2018-03-29 , DOI: 10.1016/j.seppur.2018.03.065
Liangliang Zhang , Shuying Wu , Yue Gao , Baochang Sun , Yong Luo , Haikui Zou , Guangwen Chu , Jianfeng Chen

In this work, the absorption performance of SO2 into calcium-based solution was studied in a rotating packed bed (RPB). Experiments were carried out to examine the effect of various operating parameters on the desulfurization efficiency, such as absorbent pH value, gravity level of RPB, gas-liquid ratio, gas treatment amount and inlet SO2 concentration. It was found that the SO2 removal efficiency increased with the increasing of absorbent pH value and RPB gravity level, and decreased with the increasing of the gas-liquid ratio and inlet SO2 concentration. SO2 removal efficiency was about 88% for the metal packing and 82% for the plastic packing under the optimal operating conditions when the SO2 inlet concentration was 900 mg/m3. Moreover, volumetric mass transfer coefficient (KGa) in RPB of this absorption process was calculated. It was found that KGa was 7.83–19.34 s−1 in RPB, almost 1 order of magnitude higher than that in packed tower and impinging stream gas-liquid reactor.



中文翻译:

旋转填充床中钙基溶液对SO 2的吸收

在这项工作中,在旋转填充床(RPB)中研究了SO 2在钙基溶液中的吸收性能。进行实验以检验各种操作参数对脱硫效率的影响,例如吸收剂的pH值,RPB的重力水平,气液比,气体处理量和入口SO 2浓度。结果表明,随着吸收剂pH值和RPB比重的增加,SO 2的去除效率增加;随着气液比和进口SO 2浓度的增加,SO 2的去除效率降低。在最佳操作条件下,当SO填充时,金属填充物的SO 2去除效率约为88%,塑料填充物的SO 2去除效率约为82%。2入口浓度为900 mg / m 3。另外,算出该吸收工序的RPB中的体积传质系数(K G a)。结果发现,RPB中的K g a为7.83-19.34 s -1,比填料塔和撞击流气液反应器的K G a高近1个数量级。

更新日期:2018-03-29
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