Tailoring Interfacial Nanoparticle Organization through Entropy,Accounts of Chemical Research

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Tailoring Interfacial Nanoparticle Organization through Entropy
Accounts of Chemical Research ( IF 16.4 ) Pub Date : 2018-03-28 00:00:00 , DOI: 10.1021/acs.accounts.8b00001
Guolong Zhu ₁ , Zihan Huang ₁ , Ziyang Xu ₁ , Li-Tang Yan ₁

Affiliation

The ability to tailor the interfacial behaviors of nanoparticles (NPs) is crucial not only for the design of novel nanostructured materials with superior properties and of interest for many promising applications such as water purification, enhanced oil recovery, and innovative energy transduction, but also for a better insight into many biological systems where nanoscale particles such as proteins or viruses can interact and organize at certain interfaces. As a class of emerging building blocks, Janus NPs consisting of two compartments of different chemistry or polarity are ideal candidates to generate tunable and stable interfacial nanostructures because of the asymmetric nature. However, precise control over such interfacial nanostructures toward a controllable order and even responses to various external stimuli still remains a great challenge as the interfaces do not simply serve as a scaffold but rather induce complex enthalpic and entropic interactions.

中文翻译：

通过熵调整界面纳米颗粒的组织

定制纳米颗粒（NPs）界面行为的能力不仅对于设计具有优异性能的新型纳米结构材料至关重要，而且对于许多有前途的应用（例如水净化，增强的石油采收率和创新的能量转换）也具有重要意义。深入了解许多生物系统，其中蛋白质或病毒等纳米级粒子可以在某些界面相互作用和组织。作为一类新兴的构建基块，Janus NP由两个化学性质或极性不同的部分组成，是非对称性质的理想候选物，可生成可调谐和稳定的界面纳米结构。然而，

更新日期：2018-03-28

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