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Pressure effect on the magnetic properties of the half-metallic Heusler alloyCo2TiSn
Physical Review B ( IF 3.7 ) Pub Date : 2018-03-21 00:00:00 , DOI: 10.1103/physrevb.97.104414
Iduru Shigeta , Yutaro Fujimoto , Ryutaro Ooka , Yuya Nishisako , Masahito Tsujikawa , Rie Y. Umetsu , Akiko Nomura , Kunio Yubuta , Yoshio Miura , Takeshi Kanomata , Masafumi Shirai , Jun Gouchi , Yoshiya Uwatoko , Masahiko Hiroi

Precise magnetization measurements of a half-metallic ferromagnet Co2TiSn with the Heusler type structure have been carried out under pressure up to 1.27 GPa. At ambient pressure, the spontaneous magnetic moment Msexp and the Curie temperature TCexp are experimentally obtained to be 1.993(3)μB/f.u. and 376.76(7) K, respectively. The Msexp is independent of applying pressure. The TCexp decreases with the increase of pressure and the pressure derivative of the Curie temperature dTCexp/dp is estimated to be 3.15(9) K/GPa. Furthermore, the pressure effect on the electronic and magnetic properties of Co2TiSn has been theoretically investigated on the basis of first-principles density functional calculations by using the projector augmented wave method in order to evaluate the half metallicity of Co2TiSn. Both the experimental and the theoretical results under pressure reveal that Co2TiSn is half metal. The experimental results of pressure-dependent magnetic properties are finally discussed on the basis of the spin fluctuation theory for itinerant electron magnetism.

中文翻译:

压力对半金属Heusler合金Co2TiSn磁性能的影响

半金属铁磁体的精确磁化测量 有限公司2个钛锡具有Heusler型结构的设备已在高达1.27 GPa的压力下进行。在环境压力下,自发的磁矩中号s经验值 和居里温度 ŤC经验值 通过实验获得 1.9933μ/ fu和 376.767分别为K。这中号s经验值与施加压力无关。这ŤC经验值 随压力的增加和居里温度的压力导数而减小 dŤC经验值/dp 估计是 -3.159K / GPa。此外,压力对合金的电子和磁性的影响有限公司2个钛锡 在理论上根据第一原理密度函数计算,通过使用投影机增强波方法进行了研究,以评估金属的半金属性。 有限公司2个钛锡。在压力下的实验和理论结果都表明:有限公司2个钛锡是半金属。最后,基于自旋涨落理论对迭代电子磁的压力依赖性磁性能的实验结果进行了讨论。
更新日期:2018-03-21
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