In situ plasma-assisted atmospheric nitrogen fixation using water and spray-type jet plasma,Chemical Communications

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In situ plasma-assisted atmospheric nitrogen fixation using water and spray-type jet plasma
Chemical Communications ( IF 4.3 ) Pub Date : 2018-03-02 00:00:00 , DOI: 10.1039/c8cc00697k
Peng Peng _{1,

2,

3,

4} , Paul Chen _{1,

2,

3,

4} , Min Addy _{1,

2,

3,

4} , Yanling Cheng _{1,

2,

3,

4} , Yaning Zhang _{1,

2,

3,

4,

5} , Erik Anderson _{1,

2,

3,

4} , Nan Zhou _{1,

2,

3,

4} , Charles Schiappacasse _{1,

2,

3,

4} , Raymond Hatzenbeller _{1,

2,

3,

4} , Liangliang Fan _{1,

2,

3,

4} , Shiyu Liu _{1,

2,

3,

4} , Dongjie Chen _{1,

2,

3,

4} , Juer Liu _{1,

2,

3,

4} , Yuhuan Liu _{6,

7,

8} , Roger Ruan _{1,

2,

3,

4,

6}

Affiliation

In this study, a sustainable nitrogen fixation process was presented under atmospheric conditions and without introducing hydrogen or any catalyst. The novel in situ synthesis in this study used an advanced spray-type jet plasma, which significantly improved the fixation rate of nitrite, nitrate, and ammonium. Furthermore, the mechanism focusing on the co-synthesis of the abovementioned three nitrogen compounds was proposed based on the synergistic interactions between the gas-phase plasma and liquid surface dissociation.

中文翻译：

使用水和喷雾型喷射等离子体进行原位等离子体辅助的大气固氮

在这项研究中，提出了在大气条件下且不引入氢或任何催化剂的可持续固氮方法。在这项研究中，新的原位合成使用了先进的喷雾型喷射等离子体，可显着提高亚硝酸盐，硝酸盐和铵盐的固定率。此外，基于气相等离子体与液面解离的协同作用，提出了上述三种含氮化合物共合成的机理。

更新日期：2018-03-15

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