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In situ plasma-assisted atmospheric nitrogen fixation using water and spray-type jet plasma
Chemical Communications ( IF 4.3 ) Pub Date : 2018-03-02 00:00:00 , DOI: 10.1039/c8cc00697k
Peng Peng 1, 2, 3, 4 , Paul Chen 1, 2, 3, 4 , Min Addy 1, 2, 3, 4 , Yanling Cheng 1, 2, 3, 4 , Yaning Zhang 1, 2, 3, 4, 5 , Erik Anderson 1, 2, 3, 4 , Nan Zhou 1, 2, 3, 4 , Charles Schiappacasse 1, 2, 3, 4 , Raymond Hatzenbeller 1, 2, 3, 4 , Liangliang Fan 1, 2, 3, 4 , Shiyu Liu 1, 2, 3, 4 , Dongjie Chen 1, 2, 3, 4 , Juer Liu 1, 2, 3, 4 , Yuhuan Liu 6, 7, 8 , Roger Ruan 1, 2, 3, 4, 6
Affiliation  

In this study, a sustainable nitrogen fixation process was presented under atmospheric conditions and without introducing hydrogen or any catalyst. The novel in situ synthesis in this study used an advanced spray-type jet plasma, which significantly improved the fixation rate of nitrite, nitrate, and ammonium. Furthermore, the mechanism focusing on the co-synthesis of the abovementioned three nitrogen compounds was proposed based on the synergistic interactions between the gas-phase plasma and liquid surface dissociation.

中文翻译:

使用水和喷雾型喷射等离子体进行原位等离子体辅助的大气固氮

在这项研究中,提出了在大气条件下且不引入氢或任何催化剂的可持续固氮方法。在这项研究中,新的原位合成使用了先进的喷雾型喷射等离子体,可显着提高亚硝酸盐,硝酸盐和铵盐的固定率。此外,基于气相等离子体与液面解离的协同作用,提出了上述三种含氮化合物共合成的机理。
更新日期:2018-03-15
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