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Magnetic nanoparticles/PEDOT:PSS composite hole-injection layer for efficient organic light-emitting diodes†
Journal of Materials Chemistry C ( IF 5.7 ) Pub Date : 2018-02-27 00:00:00 , DOI: 10.1039/c7tc05554d
Hong Lian 1, 2, 3, 4 , Zhenyu Tang 4, 5, 6, 7 , Hongen Guo 1, 2, 3, 4 , Zheng Zhong 1, 2, 3, 4 , Jian Wu 1, 2, 3, 4 , Qingchen Dong 1, 2, 3, 4 , Furong Zhu 4, 8, 9, 10, 11 , Bin Wei 4, 5, 6, 7 , Wai-Yeung Wong 1, 2, 3, 4, 12
Affiliation  

A multifunctional solution-processed composite hole-injection layer (HIL), based on the blends of magnetic nanoparticles (NPs) Fe3O4@G–poly(3,4-ethylenedioxythiophene):poly(styrenesulfonate) (PEDOT:PSS), Fe3O4@SiO2–PEDOT:PSS and Fe3O4@Au–PEDOT:PSS, was used for application in high performance tris-(8-hydroxyquinoline) aluminum-based organic light emitting diodes (OLEDs). Compared to the control devices, a significant increase in the current efficiency of OLEDs with a composite HIL was realized, achieving maximum luminous efficiencies of 5.13 cd A−1 (Fe3O4@G–PEDOT:PSS and Fe3O4@Au–PEDOT:PSS HIL), and of 4.83 cd A−1 (Fe3O4@SiO2–PEDOT:PSS HIL), corresponding to a 35% and 38.2% increase in current efficiency, respectively. The increase in the performance of the OLEDs is attributed to the collective effects of light-scattering, localized surface plasmon resonance (LSPR) and the magnetic effect induced by the magnetic NPs in the HIL.

中文翻译:

磁性纳米颗粒/ PEDOT:PSS复合空穴注入层,用于高效有机发光二极管

基于磁性纳米粒子(NP)Fe 3 O 4 @ G–聚(3,4-乙撑二氧噻吩):聚(苯乙烯磺酸盐)(PEDOT:PSS)的混合物的多功能固溶处理复合空穴注入层(HIL ), Fe 3 O 4 @SiO 2 -PEDOT:PSS和Fe 3 O 4 @ Au-PEDOT:PSS被用于高性能的三-(8-羟基喹啉)铝基有机发光二极管(OLED)。与控制设备相比,采用复合HIL的OLED的电流效率得到了显着提高,实现了最大发光效率达5.13 cd A -1(Fe 3 O 4 @ G–PEDOT:PSS和Fe3 O 4 @ Au–PEDOT:PSS HIL)和4.83 cd A -1(Fe 3 O 4 @SiO 2 –PEDOT:PSS HIL),分别对应于电流效率提高35%和38.2%。OLED性能的提高归因于光散射,局部表面等离振子共振(LSPR)的集体效应以及HIL中磁性NP引起的磁性效应。
更新日期:2018-02-27
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