Total synthesis and absolute configuration reassignment of mollenines A and B†,Organic Chemistry Frontiers

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Total synthesis and absolute configuration reassignment of mollenines A and B†
Organic Chemistry Frontiers ( IF 5.4 ) Pub Date : 2017-12-18 00:00:00 , DOI: 10.1039/c7qo00985b
Ming-Zhong Wang _{1,

2,

3,

4,

5} , Tong-Xu Si _{1,

2,

3,

4} , Chuen-Fai Ku _{5,

6,

7,

8} , Xiao-Wan Li _{1,

2,

3,

4} , Zheng-Ming Li _{9,

10,

11,

12,

13} , Hong-Jie Zhang _{5,

6,

7,

8} , Albert S. C. Chan _{1,

2,

3,

4}

Affiliation

The first total synthesis of the indole alkaloids mollenines A and B with the diketomorpholine skeleton has been accomplished in 9 and 10 steps with an overall yield of 11.4% and 9.3%, respectively. The absolute stereochemistry of the two natural products was corrected.

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