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Radiation-induced amorphization of Langasite La3Ga5SiO14
Journal of Nuclear Materials ( IF 2.8 ) Pub Date : 2017-12-15 , DOI: 10.1016/j.jnucmat.2017.12.023
Tiankai Yao , Fengyuan Lu , Haifeng Zhang , Bowen Gong , Wei Ji , Lei Zuo , Jie Lian

Single crystals of Langasite La3Ga5SiO14 (LGS) were irradiated by 1 MeV Kr2+ ions at temperature range from 298 to 898 K in order to simulate the damage effect of neutron radiation on Langasite, a candidate sensor material proposed as high temperature and pressure sensors in nuclear reactors. The microstructure evolution of LGS as functions of irradiation dose and temperature was followed by in-situ TEM observation through electron diffraction pattern. LGS is found to be sensitive to ion beam irradiation-induced amorphization from displacive heavy ions with a low critical dose of ∼0.5 ± 0.2 dpa (neutron fluence of (1.6 ± 0.6 ) × 1019 neutrons/cm2) at room temperature. The critical amorphization temperature, Tc, is determined to be 910 ± 10 K. Under simultaneous ionizing electron (300 keV, 45 nA) and displacive heavy ion irradiations (1-MeV Kr2+ and flux of 6.25 × 1011 ions/cm2·s), LGS displayed greater stability of crystal structure against amorphization, possibly due to the electron radiation-induced recovery of displacive damage by heavy ions.



中文翻译:

辐射诱导非晶硅La 3 Ga 5 SiO 14的非晶化

用1 MeV Kr 2+离子在298至898 K的温度范围内对Langasite La 3 Ga 5 SiO 14(LGS)的单晶进行辐照,以模拟中子辐射对Langasite的破坏作用,Langasite被认为是高候选的传感器材料。核反应堆中的温度和压力传感器。LGS的微观结构随辐射剂量和温度的变化而变化,然后通过电子衍射图谱进行原位TEM观察。已发现LGS对置换性重离子的离子束辐照引起的非晶化敏感,临界剂量低至〜0.5±0.2 dpa(中子注量为(1.6±0.6)×10 19中子/ cm 2) 在室温下。临界非晶化温度Tc确定为910±10K。在同时电离电子(300 keV,45 nA)和置换重离子辐射(1-MeV Kr 2+和通量为6.25×10 11离子/ cm 2的情况下) ·s),LGS表现出更大的晶体结构稳定性,可防止非晶化,这可能是由于电子辐射引起的重离子置换损伤的恢复。

更新日期:2017-12-15
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