Imidazolium Ions with an Alcohol Substituent for Enhanced Electrocatalytic Reduction of CO2,ChemSusChem

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Imidazolium Ions with an Alcohol Substituent for Enhanced Electrocatalytic Reduction of CO2
ChemSusChem ( IF 7.5 ) Pub Date : 2017-11-22 03:56:22 , DOI: 10.1002/cssc.201701673
Lin Zhang ₁ , Nian Wu ₁ , Jichen Zhang ₁ , Yang Hu ₁ , Zhiyong Wang ₁ , Lin Zhuang ₁ , Xianbo Jin ₁

Affiliation

The secret of the N site: A propanol substituent at the N site of the imidazonium ring can bridge a hydrogen-bonding chain between the C2−H and the O of the CO₂, which enables fast proton-hoping transfer, leading to a significant decrease of the activation barrier for the reduction of CO₂ to CO in the presence of imidazolium ionic liquids as electrolyte additives with catalytic activity.

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