Metal–Organic Framework-Stabilized CO2/Water Interfacial Route for Photocatalytic CO2 Conversion,ACS Applied Materials & Interfaces

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Metal–Organic Framework-Stabilized CO2/Water Interfacial Route for Photocatalytic CO2 Conversion
ACS Applied Materials & Interfaces ( IF 8.3 ) Pub Date : 2017-11-16 00:00:00 , DOI: 10.1021/acsami.7b13900
Tian Luo _{1,

2} , Jianling Zhang ₁ , Wei Li ₂ , Zhenhong He ₁ , Xiaofu Sun ₁ , Jinbiao Shi ₁ , Dan Shao ₁ , Bingxing Zhang ₁ , Xiuniang Tan ₁ , Buxing Han ₁

Affiliation

Here, we propose a CO₂/water interfacial route for photocatalytic CO₂ conversion by utilizing a metal–organic framework (MOF) as both an emulsifier and a catalyst. The CO₂ reduction occurring at the CO₂/water interface produces formate with remarkably enhanced efficiency as compared with that in conventional solvent. The route is efficient, facile, adjustable, and environmentally benign, which is applicable for the CO₂ transformation photocatalyzed by different kinds of MOFs.

中文翻译：

金属-有机骨架稳定的CO ₂ /水界面路线，用于光催化CO ₂转化

在这里，我们提出了利用金属-有机骨架（MOF）作为乳化剂和催化剂的光催化CO ₂转化的CO ₂ /水界面途径。与常规溶剂相比，在CO ₂ /水界面处发生的CO ₂还原产生的甲酸酯具有显着提高的效率。该路线高效，简便，可调节且对环境无害，适用于不同种类的MOF光催化的CO ₂转化。

更新日期：2017-11-17

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