Direct Aryl C−H Amination with Primary Amines using Organic Photoredox Catalysis,Angewandte Chemie International Edition

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Direct Aryl C−H Amination with Primary Amines using Organic Photoredox Catalysis
Angewandte Chemie International Edition ( IF 16.1 ) Pub Date : 2017-11-13 06:18:08 , DOI: 10.1002/anie.201709523
Kaila A. Margrey ₁ , Alison Levens ₁ , David A. Nicewicz ₁

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To be direct: Described herein is the construction of C−N bonds, using primary amines, by direct C−H functionalization with an acridinium photoredox catalyst under an aerobic conditions. The method tolerates a wide variety of primary amines, including amino acids, and the regiochemistry is influenced by the arene substitution pattern. Also notable is that it can be used in a flow chemistry setup.

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