Application of Pulse Radiolysis to Mechanistic Investigations of Catalysis Relevant to Artificial Photosynthesis,ChemSusChem

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Application of Pulse Radiolysis to Mechanistic Investigations of Catalysis Relevant to Artificial Photosynthesis
ChemSusChem ( IF 7.5 ) Pub Date : 2017-10-27 02:21:17 , DOI: 10.1002/cssc.201701559
David C. Grills ₁ , Dmitry E. Polyansky ₁ , Etsuko Fujita ₁

Affiliation

Observing fleeting moments: Pulse radiolysis (PR) is a powerful technique for investigating redox transformations relevant to artificial photosynthesis, such as catalytic water oxidation and proton or CO₂ reduction. The rapid generation of powerful reducing or oxidizing species coupled with time-resolved spectroscopy in the UV/Vis to mid-IR range allows the observation of transient intermediates that are often inaccessible through other techniques.

中文翻译：

脉冲辐射分解在人工光合作用催化机理研究中的应用

观察转瞬即逝的时刻：脉冲辐射分解（PR）是研究与人工光合作用相关的氧化还原转化（例如催化水氧化和质子或CO ₂还原）的一项强大技术。快速生成强力的还原或氧化物质，再加上时间分辨光谱，可在UV / Vis到中红外范围内观察到瞬态中间体，而这些瞬态中间体通常是其他技术无法达到的。

更新日期：2017-10-27

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