Light-Driven Hydrogen Evolution by Nickel-Substituted Rubredoxin,ChemSusChem

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Light-Driven Hydrogen Evolution by Nickel-Substituted Rubredoxin
ChemSusChem ( IF 7.5 ) Pub Date : 2017-10-25 02:55:56 , DOI: 10.1002/cssc.201701627
Michael J. Stevenson _{1,

2} , Sean C. Marguet ₁ , Camille R. Schneider ₃ , Hannah S. Shafaat _{1,

3}

Affiliation

Revenge of the NiRds: An enzymatic system for light-driven hydrogen generation has been developed through covalent attachment of a ruthenium chromophore to nickel-substituted rubredoxin (NiRd). The photoinduced activity of the hybrid enzyme is significantly greater than that of a two-component system and is strongly dependent on the position of the ruthenium phototrigger relative to the active site.

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