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Source apportionment of PM10 in Delhi, India using PCA/APCS, UNMIX and PMF
Particuology ( IF 4.1 ) Pub Date : 2017-09-01 , DOI: 10.1016/j.partic.2017.05.009
Srishti Jain , S.K. Sharma , T.K. Mandal , Mohit Saxena

Source apportionment of particulate matter (PM10) measurements taken in Delhi, India between January 2013 and June 2014 was carried out using two receptor models, principal component analysis with absolute principal component scores (PCA/APCS) and UNMIX. The results were compared with previous estimates generated using the positive matrix factorization (PMF) receptor model to investigate each model’s source-apportioning capability. All models used the PM10 chemical composition (organic carbon (OC), elemental carbon (EC), water soluble inorganic ions (WSIC), and trace elements) for source apportionment. The average PM10 concentration during the study period was 249.7 ± 103.9 μg/m3 (range: 61.4–584.8 μg/m3). The UNMIX model resolved five sources (soil dust (SD), vehicular emissions (VE), secondary aerosols (SA), a mixed source of biomass burning (BB) and sea salt (SS), and industrial emissions (IE)). The PCA/APCS model also resolved five sources, two of which also included mixed sources (SD, VE, SD+SS, (SA+BB+SS) and IE). The PMF analysis differentiated seven individual sources (SD, VE, SA, BB, SS, IE, and fossil fuel combustion (FFC)). All models identified the main sources contributing to PM10 emissions and reconfirmed that VE, SA, BB, and SD were the dominant contributors in Delhi.



中文翻译:

使用PCA / APCS,UNMIX和PMF在印度德里的10号纸机的源分配

2013年1月至2014年6月在印度德里进行的颗粒物(PM 10)物源分摊是使用两种受体模型进行的,即具有绝对主成分评分(PCA / APCS)的主成分分析和UNMIX。将结果与使用正矩阵分解(PMF)受体模型生成的先前估计值进行比较,以研究每个模型的源分配能力。所有模型都使用PM 10的化学成分(有机碳(OC),元素碳(EC),水溶性无机离子(WSIC)和微量元素)进行源分配。在研究期间,PM 10的平均浓度为249.7± 103.9μg / m 3(范围:61.4–584.8μg/ m 3)。UNMIX模型解析了五个来源(土壤粉尘(SD),车辆排放物(VE),二次气溶胶(SA),生物质燃烧(BB)和海盐(SS)的混合源以及工业排放物(IE))。PCA / APCS模型还解析了五个来源,其中两个还包括混合来源(SD,VE,SD + SS,(SA + BB + SS)和IE)。PMF分析区分了七个单独的来源(SD,VE,SA,BB,SS,IE和化石燃料燃烧(FFC))。所有模型都确定了造成PM 10排放的主要来源,并再次确认VE,SA,BB和SD是德里的主要贡献者。

更新日期:2017-09-01
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