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Magnetotransport and electronic structure of EuAuSb: A candidate antiferromagnetic Dirac semimetal
Physical Review B ( IF 3.7 ) Pub Date : 2024-04-18 , DOI: 10.1103/physrevb.109.155152
D. Ram , J. Singh , S. Banerjee , A. Sundaresan , D. Samal , V. Kanchana , Z. Hossain

We have investigated the magnetic, thermodynamic, and electrical transport properties of EuAuSb single crystals as well as carrying out band structure calculations. The powder x-ray diffraction data confirm that EuAuSb crystallizes in ZrBeSi-type hexagonal structure with space group P63/mmc. The magnetic measurements reveal an antiferromagnetic (AFM) ordering in EuAuSb at TN=3.3 K. This transition is further confirmed by heat capacity and electrical resistivity data. The isothermal magnetization data saturate at low magnetic field of μ0Hsc=2.9 and μ0Hsab=3.8 T for Hc and Hc, respectively, while the magnetization along Hc displays a metamagnetic transition around μ0Hmab=0.95 T. The electrical resistivity exhibits a metallic behavior down to 35 K; after that it shows an upturn until TN due to the influence of short-range interactions. The longitudinal and transverse magnetoresistances of EuAuSb are negative (45% and 42% in 10 T at 2 K, respectively); in the high field at T40 K, they switch to a positive value above 40 K. Further, we observe a humplike anomaly in the Hall resistivity [ρxy(H)] data below TN, which is most likely a manifestation of the topological Hall effect. Our two-band model analysis of ρxy(H) data indicates both hole and electron charge carriers contribute to the electrical transport of the compound. The electronic band structure calculations reveal a Γ-centered nodal line in the absence of spin-orbit coupling (SOC). In the presence of SOC, the compound hosts the Dirac point. The Z2 invariants, in the presence of effective time-reversal and inversion symmetries, categorize this system as a nontrivial topological material. Our combined experimental and theoretical studies suggest EuAuSb to be a potential AFM topological semimetal.

中文翻译:

EuAuSb 的磁输运和电子结构:候选反铁磁狄拉克半金属

我们研究了 EuAuSb 单晶的磁性、热力学和电输运特性,并进行了能带结构计算。粉末X射线衍射数据证实EuAuSb结晶为具有空间群的ZrBeSi型六方结构63/C。磁性测量揭示了 EuAuSb 中的反铁磁 (AFM) 有序性时间=3.3 K. 热容量和电阻率数据进一步证实了这种转变。等温磁化数据在低磁场下饱和μ0HsC=2.9μ0HsA=3.8 为HCHC,而磁化强度沿HC显示周围的变磁转变μ0HA=0.95 T. 电阻率低至 35 K 时表现出金属行为;之后它呈现出好转状态,直到时间由于短程相互作用的影响。 EuAuSb 的纵向和横向磁阻均为负值(-45%-42%分别为 10 T、2 K);在高场时间40 K,它们在 40 K 以上切换到正值。此外,我们观察到霍尔电阻率出现驼峰状异常[ρXyH] 数据如下时间,这很可能是拓扑霍尔效应的体现。我们的双频带模型分析ρXyH数据表明空穴和电子载流子都有助于化合物的电传输。电子能带结构计算揭示了γ-在没有自旋轨道耦合(SOC)的情况下以中心节点线。在 SOC 存在的情况下,该化合物具有狄拉克点。这Z2在存在有效的时间反转和反演对称性的情况下,不变量将该系统归类为非平凡的拓扑材料。我们的实验和理论相结合的研究表明,EuAuSb 是一种潜在的 AFM 拓扑半金属。
更新日期:2024-04-19
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