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Role of Debye temperature in achieving large adiabatic temperature changes at cryogenic temperatures: A case study onPr2In
Physical Review B ( IF 3.7 ) Pub Date : 2024-04-17 , DOI: 10.1103/physrevb.109.l140407 Wei Liu , Franziska Scheibel , Nuno Fortunato , Imants Dirba , Tino Gottschall , Hongbin Zhang , Konstantin Skokov , Oliver Gutfleisch
Physical Review B ( IF 3.7 ) Pub Date : 2024-04-17 , DOI: 10.1103/physrevb.109.l140407 Wei Liu , Franziska Scheibel , Nuno Fortunato , Imants Dirba , Tino Gottschall , Hongbin Zhang , Konstantin Skokov , Oliver Gutfleisch
The excellent magnetic entropy change () in the temperature range of 20 77 K due to the first-order phase transition makes an intriguing candidate for magnetocaloric hydrogen liquefaction. As an equally important magnetocaloric parameter, the adiabatic temperature change () of associated with the first-order phase transition has not yet been reported. In this work, the of is obtained from heat capacity measurements: 2 K in fields of 2 T and 4.3 K in fields of 5 T. While demonstrating a that is not as impressive as its remarkable exhibits a low Debye temperature () of around 110 K. Based on these two observations, an approach that combines the mean-field and Debye models is developed to study the correlation between , one of the most important magnetocaloric parameters, and , one important property of a material. The role of in achieving large is revealed: materials with higher tend to exhibit larger , particularly in the cryogenic temperature range. This discovery explains the absence of an outstanding in and can serve as a tool for designing or searching for materials with both a large and a .
中文翻译:
德拜温度在低温下实现大绝热温度变化的作用:Pr2In 的案例研究
优异的磁熵变()在20的温度范围内77 K 由于一阶相变使得磁热氢液化的一个有趣的候选者。作为一个同样重要的磁热参数,绝热温度变化() 的与一级相变相关的现象尚未见报道。在这项工作中,的是从热容测量中获得的:2 T 场中为 2 K,5 T 场中为 4.3 K。这并不像其非凡的那样令人印象深刻表现出较低的德拜温度()约为 110 K。基于这两个观测结果,开发了一种结合平均场和德拜模型的方法来研究之间的相关性,最重要的磁热参数之一,以及,材料的一个重要属性。的作用在实现大揭示:材料具有更高往往表现出较大的,特别是在低温范围内。这一发现解释了缺乏杰出的在并且可以作为设计或搜索具有大范围材料的工具和一个。
更新日期:2024-04-17
中文翻译:
德拜温度在低温下实现大绝热温度变化的作用:Pr2In 的案例研究
优异的磁熵变()在20的温度范围内77 K 由于一阶相变使得磁热氢液化的一个有趣的候选者。作为一个同样重要的磁热参数,绝热温度变化() 的与一级相变相关的现象尚未见报道。在这项工作中,的是从热容测量中获得的:2 T 场中为 2 K,5 T 场中为 4.3 K。这并不像其非凡的那样令人印象深刻表现出较低的德拜温度()约为 110 K。基于这两个观测结果,开发了一种结合平均场和德拜模型的方法来研究之间的相关性,最重要的磁热参数之一,以及,材料的一个重要属性。的作用在实现大揭示:材料具有更高往往表现出较大的,特别是在低温范围内。这一发现解释了缺乏杰出的在并且可以作为设计或搜索具有大范围材料的工具和一个。