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Advances in carbon nitride supported single-atom photocatalysts for hydrogen evolution
Current Opinion in Chemical Engineering ( IF 6.6 ) Pub Date : 2023-06-30 , DOI: 10.1016/j.coche.2023.100941
Fanpeng Meng , Zhihao Tian , Wenjie Tian , Huayang Zhang

Owing to their distinct collaboration nature, high atom usage, and high catalytic performance, single-atom catalysts have become most dynamically studied in various catalytic reactions. Graphitic carbon nitride (g-CN), as one of the most promising two-dimensional supports for stable immobilization of single-atom metals, has received extensive investigations. In this review, the recent developments of g-CN-supported single-atom photocatalysts for hydrogen evolution are summarized, with the metal-support interactions and structure regulations for stable and efficient catalysis being highlighted. Finally, the difficulties and potentials for future development of g-CN-supported single-atom materials in photocatalytic hydrogen evolution are proposed.

中文翻译:

氮化碳负载单原子光催化剂析氢研究进展

由于其独特的协作性质、高原子利用率和高催化性能,单原子催化剂在各种催化反应中已成为最活跃的研究对象。石墨氮化碳(g-CN)作为最有前途的稳定固定单原子金属的二维载体之一,已受到广泛的研究。在这篇综述中,总结了 g-CN 负载的单原子光催化剂用于析氢的最新进展,重点介绍了金属-载体相互作用和稳定高效催化的结构调控。最后,提出了g-CN负载单原子材料在光催化析氢方面未来发展的困难和潜力。
更新日期:2023-06-30
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