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Enaminone-Linked Covalent Organic Frameworks for Boosting Photocatalytic Hydrogen Production
Angewandte Chemie International Edition ( IF 16.1 ) Pub Date : 2023-05-31 , DOI: 10.1002/anie.202306135 Xinyu Guan 1 , Yunyang Qian 1 , Xiyuan Zhang 1 , Hai-Long Jiang 1
Angewandte Chemie International Edition ( IF 16.1 ) Pub Date : 2023-05-31 , DOI: 10.1002/anie.202306135 Xinyu Guan 1 , Yunyang Qian 1 , Xiyuan Zhang 1 , Hai-Long Jiang 1
Affiliation
The enaminone-linked COFs (En-COFs) are synthesized and firstly attempted for photocatalysis. Compared with the corresponding imine-linked COFs (Im-COFs) and quinoline-linked COFs (Qu-COFs) with almost identical structures but altered linkages, En-COFs possess boosted photocatalytic activity with extended light adsorption, facilitated exciton dissociation and improved stability, making them a promising platform for enhanced photocatalysis.
中文翻译:
用于促进光催化产氢的烯胺酮连接的共价有机框架
合成了烯胺酮连接的 COF(En-COF)并首次尝试用于光催化。与结构几乎相同但连接方式不同的相应亚胺连接的COF(Im-COF)和喹啉连接的COF(Qu-COF)相比,En-COF具有增强的光催化活性、延长的光吸收、促进激子解离和提高的稳定性。使它们成为增强光催化的有前途的平台。
更新日期:2023-05-31
中文翻译:
用于促进光催化产氢的烯胺酮连接的共价有机框架
合成了烯胺酮连接的 COF(En-COF)并首次尝试用于光催化。与结构几乎相同但连接方式不同的相应亚胺连接的COF(Im-COF)和喹啉连接的COF(Qu-COF)相比,En-COF具有增强的光催化活性、延长的光吸收、促进激子解离和提高的稳定性。使它们成为增强光催化的有前途的平台。