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Organic thin-film transistors with sub-10-micrometer channel length with printed polymer/carbon nanotube electrodes
Organic Electronics ( IF 2.7 ) Pub Date : 2017-10-20 , DOI: 10.1016/j.orgel.2017.10.023
So Hyun Park , Jiye Kim , Seungyoung Lee , Dong Yun Lee , Sooman Lim , Jaewoong Lee , Se Hyun Kim

An electrohydrodynamic (EHD) jet printing technique was used for direct printing of a conductive polymer combined with carbon nanotubes (CNT). The solutions mixture of poly(3,4-ethylenedioxythiophene):poly(4-styrenesulfonate) (PEDOT:PSS) and carbon nanotubes (CNTs) wrapped with PSS served as a PEDOT:PSS/CNT composite ink for the EHD jet printing. The EHD jet-printed patterns of the PEDOT:PSS/CNT composite exhibited excellent dimensional stability and provided sub-10-micrometer channel lengths suitable for highly integrated organic thin-film transistors (OTFTs). The resulting pentacene OTFTs employing the channel length of 7 μm yielded the field-effect mobility of 0.03 ± 0.01 cm2/(V s). In addition, we investigated the electronic structure and the crystalline morphology at the interface between pentacene and the PEDOT:PSS/CNT composite electrode, as well as the contact resistance of the OTFTs by varying the channel length produced by the EHD jet printing process.



中文翻译:

沟道长度小于10微米的有机薄膜晶体管,带有印刷的聚合物/碳纳米管电极

电液动力学(EHD)喷射印刷技术用于直接印刷与碳纳米管(CNT)结合的导电聚合物。聚(3,4-乙撑二氧噻吩):聚(4-苯乙烯磺酸盐)(PEDOT:PSS)和包裹有PSS的碳纳米管(CNT)的溶液混合物用作EHD喷墨印刷的PEDOT:PSS / CNT复合油墨。PEDOT:PSS / CNT复合材料的EHD喷墨印刷图案具有出色的尺寸稳定性,并提供了小于10微米的沟道长度,适用于高度集成的有机薄膜晶体管(OTFT)。通道长度为7μm的并五苯OTFT的场效应迁移率为0.03±0.01 cm 2/(V s)。此外,我们通过改变EHD喷射印刷工艺产生的沟道长度,研究了并五苯与PEDOT:PSS / CNT复合电极之间界面的电子结构和晶体形态,以及OTFT的接触电阻。

更新日期:2017-10-20
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