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Two-dimensional metal–organic frameworks with high oxidation states for efficient electrocatalytic urea oxidation
Chemical Communications ( IF 4.3 ) Pub Date : 2017-09-13 00:00:00 , DOI: 10.1039/c7cc06378d
Dongdong Zhu 1, 2, 3, 4 , Chunxian Guo 1, 2, 3, 4 , Jinlong Liu 1, 2, 3, 4 , Liang Wang 4, 5, 6, 7 , Yi Du 4, 5, 6, 7 , Shi-Zhang Qiao 1, 2, 3, 4
Affiliation  

A two-dimensional metal–organic framework (MOF) comprising nickel species and an organic ligand of benzenedicarboxylic acid is fabricated and explored as an electrocatalyst for urea oxidation reaction (UOR). The excellent UOR performance is found to be partially due to the high active site density of the two-dimensional MOF, and largely because of the high oxidation state of the nickel species.

中文翻译:

具有高氧化态的二维金属-有机骨架,可有效地电催化尿素氧化

制备并研究了由镍物种和苯二甲酸的有机配体组成的二维金属有机骨架(MOF),并将其用作尿素氧化反应(UOR)的电催化剂。发现优异的UOR性能部分归因于二维MOF的高活性位点密度,并且很大程度上归因于镍物质的高氧化态。
更新日期:2017-09-20
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