Two-dimensional metal–organic frameworks with high oxidation states for efficient electrocatalytic urea oxidation,Chemical Communications

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Two-dimensional metal–organic frameworks with high oxidation states for efficient electrocatalytic urea oxidation
Chemical Communications ( IF 4.3 ) Pub Date : 2017-09-13 00:00:00 , DOI: 10.1039/c7cc06378d
Dongdong Zhu _{1,

2,

3,

4} , Chunxian Guo _{1,

2,

3,

4} , Jinlong Liu _{1,

2,

3,

4} , Liang Wang _{4,

5,

6,

7} , Yi Du _{4,

5,

6,

7} , Shi-Zhang Qiao _{1,

2,

3,

4}

Affiliation

A two-dimensional metal–organic framework (MOF) comprising nickel species and an organic ligand of benzenedicarboxylic acid is fabricated and explored as an electrocatalyst for urea oxidation reaction (UOR). The excellent UOR performance is found to be partially due to the high active site density of the two-dimensional MOF, and largely because of the high oxidation state of the nickel species.

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