The role of various oxygen species in Mn-based layered double hydroxide catalysts in selective alcohol oxidation,Catalysis Science & Technology

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The role of various oxygen species in Mn-based layered double hydroxide catalysts in selective alcohol oxidation
Catalysis Science & Technology ( IF 4.4 ) Pub Date : 2017-09-07 00:00:00 , DOI: 10.1039/c7cy00918f
Yiyun Du _{1,

2,

3,

4} , Qian Wang _{1,

2,

3,

4} , Xiao Liang _{1,

2,

3,

4} , Pengfei Yang _{1,

2,

3,

4} , Yufei He _{1,

2,

3,

4} , Junting Feng _{1,

2,

3,

4} , Dianqing Li _{1,

2,

3,

4}

Affiliation

Precise identification of oxygen species in LDH-based catalysts was investigated for the first time for alcohol oxidation. Assisted by surface O²⁻, O₂ molecules were activated in various oxidation states. Labile oxygen species could react with alcohol except for the O₂²⁻ immobilized by unsaturated metals, while other oxygen species only transferred oxygen species as mediators.

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