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Fully Solution‐Processed TCO‐Free Semitransparent Perovskite Solar Cells for Tandem and Flexible Applications
Advanced Energy Materials ( IF 24.4 ) Pub Date : 2017-09-01 , DOI: 10.1002/aenm.201701569
Yaokang Zhang 1 , Zhongwei Wu 1 , Peng Li 1 , Luis K. Ono 2 , Yabing Qi 2 , Jixiang Zhou 3, 4 , Hui Shen 3 , Charles Surya 4 , Zijian Zheng 1
Affiliation  

Semitransparent perovskite solar cells (st‐PSCs) have received remarkable interest in recent years because of their great potential in applications for solar window, tandem solar cells, and flexible photovoltaics. However, all reported st‐PSCs require expensive transparent conducting oxides (TCOs) or metal‐based thin films made by vacuum deposition, which is not cost effective for large‐scale fabrication: the cost of TCOs is estimated to occupy ≈75% of the manufacturing cost of PSCs. To address this critical challenge, this study reports a low‐temperature and vacuum‐free strategy for the fabrication of highly efficient TCO‐free st‐PSCs. The TCO‐free st‐PSC on glass exhibits 13.9% power conversion efficiency (PCE), and the four‐terminal tandem cell made with the st‐PSC top cell and c‐Si bottom cell shows an overall PCE of 19.2%. Due to the low processing temperature, the fabrication of flexible st‐PSCs is demonstrated on polyethylene terephthalate and polyimide, which show excellent stability under repeated bending or even crumbing.

中文翻译:

完全解决方案处理的无TCO的半透明钙钛矿太阳能电池,适用于串联和灵活应用

近年来,半透明钙钛矿太阳能电池(st-PSC)引起了人们的极大兴趣,因为它们在太阳能窗口,串联太阳能电池和柔性光伏应用中具有巨大的潜力。但是,所有报道的st-PSC都需要昂贵的透明导电氧化物(TCO)或通过真空沉积制成的金属基薄膜,这对于大规模制造而言并不划算:估计TCO的成本约占总成本的75%。 PSC的制造成本。为了应对这一关键挑战,本研究报告了一种用于制造高效无TCO st-PSC的低温和无真空策略。玻璃上不含TCO的st-PSC表现出13.9%的功率转换效率(PCE),而由st-PSC顶部电池和c-Si底部电池制成的四端串联电池的整体PCE为19.2%。
更新日期:2017-09-01
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