Carbon dioxide-to-methanol single-pot conversion using a C-scorpionate iron(II) catalyst,Green Chemistry

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Carbon dioxide-to-methanol single-pot conversion using a C-scorpionate iron(II) catalyst
Green Chemistry ( IF 9.3 ) Pub Date : 2017-08-30 00:00:00 , DOI: 10.1039/c7gc01993a
A. P. C. Ribeiro _{1,

2,

3,

4,

5} , L. M. D. R. S. Martins _{1,

2,

3,

4,

5} , A. J. L. Pombeiro _{1,

2,

3,

4,

5}

Affiliation

The highly efficient eco-friendly synthesis of methanol (44% yield, TONs up to 2.3 × 10³) directly from carbon dioxide is achieved by using H₂ and the iron(II) scorpionate catalyst [FeCl₂{κ³-HC(pz)₃}] (pz = pyrazol-1-yl) in a solvent- or amine-free mild new protocol.

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