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Plasma technology – a novel solution for CO2 conversion?
Chemical Society Reviews ( IF 40.4 ) Pub Date : 2017-08-21 00:00:00 , DOI: 10.1039/c6cs00066e
Ramses Snoeckx 1, 2, 3, 4, 5 , Annemie Bogaerts 1, 2, 3, 4, 5
Affiliation  

CO2 conversion into value-added chemicals and fuels is considered as one of the great challenges of the 21st century. Due to the limitations of the traditional thermal approaches, several novel technologies are being developed. One promising approach in this field, which has received little attention to date, is plasma technology. Its advantages include mild operating conditions, easy upscaling, and gas activation by energetic electrons instead of heat. This allows thermodynamically difficult reactions, such as CO2 splitting and the dry reformation of methane, to occur with reasonable energy cost. In this review, after exploring the traditional thermal approaches, we have provided a brief overview of the fierce competition between various novel approaches in a quest to find the most effective and efficient CO2 conversion technology. This is needed to critically assess whether plasma technology can be successful in an already crowded arena. The following questions need to be answered in this regard: are there key advantages to using plasma technology over other novel approaches, and if so, what is the flip side to the use of this technology? Can plasma technology be successful on its own, or can synergies be achieved by combining it with other technologies? To answer these specific questions and to evaluate the potentials and limitations of plasma technology in general, this review presents the current state-of-the-art and a critical assessment of plasma-based CO2 conversion, as well as the future challenges for its practical implementation.

中文翻译:

等离子体技术–一种新颖的CO 2转化解决方案?

将CO 2转化为增值化学品和燃料被认为是21世纪的一大挑战。由于传统热方法的局限性,正在开发几种新颖的技术。等离子技术是该领域中迄今很少受到关注的一种有前途的方法。它的优点包括运行条件温和,易于升级,通过高能电子而不是热量激活气体。这允许发生热力学上困难的反应,例如CO 2裂解和甲烷的干重整,以合理的能源成本进行。在这篇综述中,在探索了传统的热学方法之后,我们简要概述了各种新颖方法之间的激烈竞争,以期找到最有效,最高效的CO 2。转换技术。需要严格评估等离子体技术在已经拥挤的舞台上能否成功。在这方面需要回答以下问题:与其他新颖方法相比,使用等离子体技术是否有主要优势?如果是,使用该技术的反面是什么?等离子体技术能否成功获得成功,还是可以通过将其与其他技术相结合来实现协同作用?为了回答这些特定问题并总体上评估等离子体技术的潜力和局限性,本综述介绍了基于等离子体的CO 2转化的当前最新技术和关键评估,以及其未来面临的挑战实际执行。
更新日期:2017-08-22
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