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Wavelength dependence of high-harmonic yield in stretched molecules
Chemical Physics ( IF 2.3 ) Pub Date : 2017-06-11 00:00:00 , DOI: 10.1016/j.chemphys.2017.05.021
Shengjun Yue , Hongchuan Du , Hongmei Wu , Jinbin Li , Bitao Hu

We study the wavelength dependence of harmonic yield in stretched molecules. It is found that when the laser field is perpendicular to the molecular axis, the harmonic yield has a slow scaling λ-4.27 as the increase of the laser wavelength for the stretched molecule View the MathML source with the internuclear distance of 7 a.u. compared with λ-5.11 for View the MathML source at the equilibrium position. Further analysis shows that the narrower width of the initial wave-function in the momentum space is in charge of the slow wavelength scaling of the stretched molecule since it can make the wave-function spreading less during propagation. Moreover, a higher enhancement and a better wavelength scaling of harmonic yield both can be achieved at the optimal internuclear distance of 7 a.u..

中文翻译:

拉伸分子中高谐波产量的波长依赖性

我们研究了拉伸分子中谐波产量的波长依赖性。发现当激光场垂直于分子轴时,谐波产量具有缓慢的缩放λ- 4.27 随着被拉伸分子的激光波长的增加 查看MathML源核间距为7 au与λ- 5.11比较 为了 查看MathML源在平衡位置。进一步的分析表明,动量空间中初始波函数的较窄宽度负责拉伸分子的慢波长缩放,因为它可以使波函数在传播过程中扩展较少。而且,在7 au的最佳核间距下,都可以实现更高的增强和更好的谐波产量的波长定标。
更新日期:2017-06-27
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