Tsang, SC Edman - University of Oxford - Department of Chemistry

研究领域

Welcome to the Tsang group at the University of Oxford. Our research is on both fundamental and applied aspects in Novel Chemistry Materials and Catalysis; Work involves synthesis, testing and characterisation of novel solid state materials for a wide range of applications particularly in the areas of catalysis, sensor and bio-medicine. Uses of well-defined single atoms, layer structures or nanomaterials as building blocks for synthesis of functional materials including development of novel core-shell nanoparticles, 2-D layers of controllable composition, size and morphology as new nanocatalysts; hollow carbon nanotubes as a nano-scale test tube for separation, storage, magnetic and electronic applications; immobilized biomolecules on nanoparticles as new sensors, etc. In the catalysis area, we work on new catalytic techniques for sustainable energy systems (fuel cells catalysts, photocatalytic solar cells, biomasses to fuel conversion, wind-to-ammonia, hydrogen storage, cleaner catalytic combustion, carbon dioxide activation, capture, storage and subsequent conversion into useful chemicals/materials (reduction in carbon emissions), etc.

近期论文

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Molecular nitrogen promotes catalytic hydrodeoxygenation Duan et. al., Nat Catal. 2019, doi:10.1038/s41929-019-0368-6. Differential adsorption of L- and D-lysine on achiral MFI zeolites as determined by synchrotron X-ray powder diffraction and thermogravimetric analysis Chen, B. Huang, S. Day, C. C. Tang, S.C.E. Tsang, KY Wong, T.W. B. Lo, Angewante Chemie 2019, doi.org/10.1002/anie.201909352. Efficient Non-dissociative Activation of Dinitrogen to Ammonia over Lithium-Promoted Ruthenium Nanoparticles at Low Pressure Zheng, F. Liao, S. Wu, G. Jones, T-Y. Chen, J. Fellowes, T. Sudmeier, I. J. McPherson, I. Wilkinson, and S. C. E. Tsang, Angewante Chemie 2019, doi.org/10.1002/anie.201907171. The Feasibility of Electrochemical Ammonia Synthesis in Molten LiCl-KCl Eutectics J. McPherson, T. Sudmeier, J. P. Fellowes, I. Wilkinson, T. Hughes, and S. C. E. Tsang, Angewante Chemie 2019, doi.org/ 10.1002/anie.201909831. Selective Production of Diethyl Maleate via Oxidative Cleavage of Lignin Aromatic Unit Zhenping Cai, Jinxing Long, Yingwen Li, Lin Ye, Biaolin Yin, Liam John France, Juncai Dong, Lirong Zheng, Hongyan He, Sijie Liu, Shik Chi Edman Tsang, Xuehui Li, 2019, doi.org/10.1016/j.chempr.2019.05.021. Photocatalytic water splitting by N-TiO2 on MgO (111) with exceptional quantum efficiencies at elevated temperatures Li, Y-K Peng, L. Hu, J. Zheng, D. Prabhakaran, S. Wu, T. J. Puchtler, M. Li, K-Y. Wong, R. A. Taylor, S. C. E. Tsang, Nat. Comm. 2019 /doi.org/10.1038/s41467-019-12385-1. Self- Regeneration of Au/CeO2 based Catalysts with Enhanced Activity and Ultra-stability for Acetylene Hydrochlorination Lin Ye, Xinping Duan, Simson Wu, Tai-Sing Wu, Yuxin Zhao, Alex W. Robertson, Hung-Lung Chou, Jianwei Zheng,Tuğçe Ayvali, Sarah Day, Chiu Tang, Yun-Liang Soo, Youzhu Yuan and Shik Chi Edman Tsang, Nat. Comm. 2019 /doi.org/10.1038/s41467-019-08827-5. Structural flexibility of a metal-organic framework induced by CO2 migration in its non-uniform porous structure Pu Zhao, Hong Fang, Sanghamitra Mukhopadhyay, Aurelia Li, Svemir Rudić, Ian J. McPherson, Chiu C. Tang, David Fairen-Jimenez, S. C. Edman Tsang and Simon A. T. Redfern, Nat. Comm. 2019, /doi.org/10.1038/s41467-019-08939-y. Engineering Monolayer 1T-MoS2 into a Bifunctional Electrocatalyst via Sonochemical Doping of Isolated Transition Metal Atoms H. M. Lau, S. Wu, R. Kato, T-S. Wu, J. Kulhavý, J. Mo, J. Zheng, J. S. Foord, Y-L. Soo, K. Suenaga, M. T. Darby, S. C. E. Tsang, ACS Catal. 2019, 9, 8, 7527-7534. Ceria Nanocrystals Supporting Pd for Formic Acid Electrocatalytic Oxidation: Prominent Polar Surface Metal Support Interactions Ye, A. H. Mahadi, C. Saengruengrit, J. Qu, F. Xu, S. M. Fairclough, N. Young, P-L Ho, J. Shan, L. Nguyen, F. F. Tao, K. Tedsree and S. C. E. Tsang, ACS Catal. 2019, 9, 6, 5171-5177. Superior Performance of Ag over Pt for Hydrogen Evolution Reaction in Water Electrolysis under High Overpotentials, J Mo, B.I. Stefanov, T.H.M. Lau, T. Chen, S. Wu, Z. Wang, X.Q. Gong, I. Wilkinson and S. C. E. Tsang, ACS Applied Energy Materials 2019, 2 (2), 1221-1228. Monitoring the methanol conversion process in H-ZSM-5 using synchrotron X-ray powder diffraction-mass spectrometry B.T.W. Lo, L. Ye, C.A. Murray, C.C. Tang, D. Mei, S.C.E. Tsang, Journal of Catalysis, 365,145-152, 2018. Carbon nitrides and metal nanoparticles: from controlled synthesis to design principles for improved photocatalysis, I.F. Teixeira, E.C.M. Barbosa, S.C.E. Tsang , P. H. C. Camargo Chem. Soc. Rev., 10.1039/C8CS00479J, 2018, Advance Article. Entrapped Single Tungstate Site in Zeolite for Cooperative Catalysis of Olefin Metathesis with Brønsted Acid Site Pu Zhao†, Lin Ye†, Zhenyu Sun, Benedict T.W. Lo, Harry Woodcock, Chen Huang, Chiu Tang, Angus I. Kirkland, Donghai Mei, and Shik Chi Edman Tsang. J. Am. Chem. Soc., DOI: 10.1021/jacs.8b03012. 2018 Transition Metal Atom Doping of the Basal Plane of MoS2 Monolayer Nanosheets for Electrochemical Hydrogen Evolution Thomas H.M Lau, XiaoWei Lu, Jiří Kulhavý, Simson Wu, Lilin Lu, Tai-Sing Wu, Ryuichi Kato, John S. Foord, Yun-Liang Soo, Kazu Suenaga, and Shik Chi Edman Tsang. Chem. Sci., DOI: 10.1039/C8SC01114A, 2018. Dynamic Modification of Pore Opening of SAPO-34 by Adsorbed Surface Methoxy Species during Induction of Catalytic Methanol-to-Olefins Reactions, B.T.W. Lo, L. Ye, G.G.Z. Chang, K. Purchase, S. Day, C.C. Tang, D. Mei, S.C.E. Tsang, Appl. Catal. B:, 237, 245-250, 2018. The Contribution of Synchrotron Powder X-ray Diffraction to Modern Zeolite Catalytic Applications: A Mini-review and Future Prospects B. Lo†, L. Ye†, S.C.E. Tsang, CHEM, accepted, 2018. Reaction: “Green” Ammonia Production, L. Ye, R. Nayak-Luke, R. Bañares-Alcántara, E. Tsang, CHEM, doi.org/10.1016/j.chempr.2017.10.016, 2017. Bimetallic Catalysts for Green Methanol Production via CO2 and Renewable Hydrogen: A Mini-review and Prospects, Molly Meng-Jung Li and Shik Chi Edman Tsang, Catal. Sci. Technol., 8, 3450-3464, 2018. CO2 Hydrogenation to Methanol over Catalysts Derived from Single Cationic Layer CuZnGa LDH Precursors Molly M.-J. Li, Chunping Chen, Tuğçe Ayvalı, Hongri Suo, Jianwei Zheng, Ivo F. Teixeira, Lin Ye, Hanbo Zou, Dermot O’Hare and Shik Chi Edman Tsang, ACS Catal. 8, 4390−4401, 2018.