Saines, Paul - University of Oxford - Department of Chemistry

研究领域

Many modern technologies are underpinned by materials with complex and tuneable electronic and magnetic interactions. Optimising these properties requires the creation of novel functional compounds and our work focuses on designing new coordination compounds that form extended crystalline frameworks. The unusual architectures of these materials are controlled by the cations and ligands they incorporate. Their useful electronic and magnetic behaviour are intricately linked to their crystal structures and we use cutting-edge characterisation techniques to facilitate the development of materials with enhanced properties via an understanding of their structure-property relationship

近期论文

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(1) Saines, P. J.; Barton P. T.; Jura, M.; Knight; K. S.; Cheetham, A. K.: Cobalt Adipate, Co(C6H8O4): Antiferromagnetic Structure, Unusual Thermal Expansion and Magnetoelastic Coupling. Mater. Horiz. 2014 Kalaji, A.; Saines P. J.; George, N. C.; Cheetham A. K.: Photoluminescence of cerium-doped (Ca1−xSrx)3RE2Ge3O12 garnet phosphors for solid state lighting: Relating structure to emission. Chem. Phys. Lett. 2013, 586, 91. Saines P. J.; Tucker, M. G.; Keen, D. A.; Cheetham, A. K.; Goodwin, A. L.: Coupling of the local defect and magnetic structure of Wüstite, Fe1–xO. Phys. Rev. B 2013, 88, 134418. Li, W.; Zhang, Z.; Bithell, E. G.; Batsanov, A. S.; Barton, P. T.; Saines, P. J.; Jain, P.; Howard, C. J.; Carpenter, M. A.; Cheetham, A. K.: Ferroelasticity in a metal-organic framework perovskite; towards a new class of multiferroics. Acta Mater. 2013, 61, 4928. Bennett, T. D.; Saines, P. J.; Keen, D. A.; Tan, J.-C.; Cheetham, A. K.: Ball-Milling-Induced Amorphization of Zeolitic Imidazolate Frameworks (ZIFs) for the Irreversible Trapping of Iodine. Chem. Eur. J. 2013, 19, 7049. Yeung, H. H. M.; Li, W.; Saines, P. J.; Koester, T. K. J.; Grey, C. P.; Cheetham, A. K.: Ligand-Directed Control over Crystal Structures of Inorganic-Organic Frameworks and Formation of Solid Solutions. Angew. Chem., Int. Ed. 2013, 52, 5544. Saines, P. J.; Steinmann, M.; Tan, J.-C.; Yeung, H. H. M.; Cheetham, A. K.: Structural diversity and luminescent properties of lanthanide 2,2- and 2,3-dimethylsuccinate frameworks. CrystEngComm 2013, 15, 100. Klintberg, L. E.; Goh, S. K.; Alireza, P. L.; Saines, P. J.; Tompsett, D. A.; Logg, P. W.; Yang, J.; Chen, B.; Yoshimura, K.; Grosche, F. M.: Pressure- and composition-induced structural quantum phase transition in the cubic superconductor (Sr, Ca)3Ir4Sn13. Phys. Rev. Lett. 2012, 109, 237008. Saines, P. J.; Steinmann, M.; Tan, J.-C.; Yeung, H. H. M.; Li, W.; Barton, P. T.; Cheetham, A. K.: Isomer-Directed Structural Diversity and Its Effect on the Nanosheet Exfoliation and Magnetic Properties of 2,3-Dimethylsuccinate Hybrid Frameworks. Inorg. Chem. 2012, 51, 11198. Zhang, Z.; Church, N.; Lappe, S.-C.; Reinecker, M.; Fuith, A.; Saines, P. J.; Harrison, R. J.; Schranz, W.; Carpenter, M. A.: Elastic and anelastic anomalies associated with the antiferromagnetic ordering transition in wustite, FexO. J. Phys.: Condens. Mat. 2012, 24, 215404. Saines, P. J.; Tan, J.-C.; Yeung, H. H. M.; Barton, P. T.; Cheetham, A. K.: Layered inorganic-organic frameworks based on the 2,2-dimethylsuccinate ligand: structural diversity and its effect on nanosheet exfoliation and magnetic properties. Dalton Trans. 2012, 41, 8585. Saines, P. J.; Barton, P. T.; Jain, P.; Cheetham, A. K.: Structures and magnetic properties of Mn and Co inorganic-organic frameworks with mixed linear dicarboxylate ligands. CrystEngComm 2012, 14, 2711. Tan, J.-C.; Saines, P. J.; Bithell, E. G.; Cheetham, A. K.: Hybrid Nanosheets of an Inorganic-Organic Framework Material: Facile Synthesis, Structure, and Elastic Properties. ACS Nano 2012, 6, 615. Saines, P. J.; Jain, P.; Cheetham, A. K.: Evolution of the structures and magnetic properties of the manganese dicarboxylates, Mn2(CO2(CH2)nCO2)(OH)2 and Mn4(CO2(CH2)nCO2)3(OH)2. Chem. Sci. 2011, 2, 1929. Saines, P. J.; Yeung, H. H. M.; Hester, J. R.; Lennie, A. R.; Cheetham, A. K.: Detailed investigations of phase transitions and magnetic structure in Fe(III), Mn(II), Co(II) and Ni(II) 3,4,5-trihydroxybenzoate (gallate) dihydrates by neutron and X-ray diffraction. Dalton Trans. 2011, 40, 6401. Saines, P. J.; Hester, J. R.; Cheetham, A. K.: Neutron diffraction study of the magnetic structures of manganese succinate Mn(C4H4O4): A complex inorganic-organic framework. Phys. Rev. B 2010, 82, 144435. Saines, P. J.; Melot, B. C.; Seshadri, R.; Cheetham, A. K.: Synthesis, Structure and Magnetic Phase Transitions of the Manganese Succinate Hybrid Framework, Mn(C4H4O4). Chem. Eur. J. 2010, 16, 7579.