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个人简介

Staff Scientist, The Molecular Foundry, LBNL, 2005–2007 Postdoctoral Fellow, IBM T. J. Watson Research Center, 2003–2005 University of Hamburg, Germany, Ph.D., 2002 Belarusian State University, Diploma 1996

研究领域

Nanocrystals in Molten Salts Our group recently reported on the formation of colloidal solutions of NCs dispersed in molten inorganic salts. Molten inorganic salts represent a very attractive class of solvents for the synthesis and processing of nanomaterials due to their high temperature stability, wide electrochemical window, stability in the presence of highly reactive species, the ability to dissolve many ionic solids not soluble in traditional solvents, and transparency in a broad range of the electromagnetic spectrum. Currently we explore both fundamental and applied aspects of these unusual colloidal media. State-Resolved Charge Transport in Colloidal Quantum Dots The novel hybrid surface passivation process efficiently eliminates surface states of HgTe QDs, enabling reversible filling of quantum-confined orbitals, switching between n-type and p-type transport, and air-stable tunable doping. The striking observations of well-resolved conductance peaks for the HgTe QD FETs and unprecedentedly high electron mobility for QD devices showing transport through discrete electronic states, represent a new level of control and performance in the application of QD solids. Direct Optical Patterning of Inorganic Materials We introduced a general chemical approach for photoresist-free, direct optical lithography of functional inorganic nanomaterials (DOLFIN). The patterned materials can be metals, semiconductors, oxides, magnetic, or rare earth compositions. No organic impurities are present in the patterned layers, which helps achieve good electronic and optical properties.

近期论文

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Composition-defined Optical Properties and the Direct to Indirect Transition in Core-Shell In1–xGaxP/ZnS Colloidal Quantum Dots Aritrajit Gupta, Justin C. Ondry, Kailai Lin, Yunhua Chen, Margaret H. Hudson, Min Chen, Richard D. Schaller, Aaron J. Rossini, Eran Rabani and Dmitri V. Talapin. Accepted for publication in Journal of the American Chemical Society. Hybrid organic-inorganic two-dimensional metal carbide MXenes with amido- and imido-terminated surfaces Chenkun Zhou, Di Wang, Francisco Lagunas, Benjamin Atterberry, Ming Lei, Huicheng Hu, Zirui Zhou, Alexander S. Filatov, De-en Jiang, Aaron J. Rossini, Robert F. Klie and Dmitri V. Talapin. Accepted for publication in Nature Chemistry. High-efficiency stretchable light-emitting polymers from thermally activated delayed fluorescence W.i Liu, Cheng Zhang, Riccardo Alessandri, Benjamin T. Diroll, Yang Li, Heyi Liang, Xiaochun Fan, Kai Wang, Himchan Cho, Youdi Liu, Yahao Dai, Qi Su, Nan Li, Songsong Li, Shinya Wai, Qiang Li, Shiyang Shao, Lixiang Wang, Jie Xu, Xiaohong Zhang, Dmitri V. Talapin, Juan J. de Pablo and Sihong Wang. Accepted to Nature Materials. Understanding and controlling photothermal responses in MXenes B.rak Guzelturk, Vladislav Kamysbayev, Di Wang, Huicheng Hu, Ruiyu Li, Sarah B. King, Alexander H. Reid, Ming-Fu Lin, Xijie Wang, Donald A. Walko, Xiaoyi Zhang, Aaron M. Lindenberg, and Dmitri V. Talapin. Accepted to Nano Letters. Excitonic Spin-Coherence Lifetimes in CdSe Nanoplatelets Increase Significantly with Core/Shell Morphology Phillip I. Martin, Shobhana Panuganti, Joshua C. Portner, Nicolas E. Watkins, Mercouri G. Kanatzidis, Dmitri V. Talapin, and Richard D. Schaller. Nano Letters 2023, 23, 4, 1467-1473 Design rules for obtaining narrow luminescence from semiconductors made in solution Hao A. Nguyen, Grant Dixon, Florence Y. Dou, Shaun Gallagher, Stephen Gibbs, Dylan Ladd, Emanuele Marino, Justin C. Ondry, James P. Shanahan, Eugenia S. Vasileiadou, Stephen Barlow, Daniel R. Gamelin, David S. Ginger, David Jonas, Mercouri G. Kanatzidis, Seth R. Marder, Daniel Morton, Christopher B. Murray, Jonathan S. Owen, Dmitri V. Talapin, Michael F. Toney, and Brandi M. Cossairt. Chemrxiv preprint. Direct synthesis and chemical vapor deposition of 2D carbide and nitride MXenes Di Wang, Chenkun Zhou, Alexander S. Filatov, Wooje Cho, Francisco Lagunas, Mingzhan Wang, Suriyanarayanan Vaikuntanathan, Chong Liu, Robert F. Klie, and Dmitri V. Talapin. Science 2023, 379, 6638, 1242-1247 (Cover article) Synthesis of Colloidal GaN and AlN Nanocrystals in Biphasic Molten Salt/Organic Solvent Mixtures under High-Pressure Ammonia W.oje Cho, Zirui Zhou, Ruiming Lin, Justin C. Ondry, and Dmitri V. Talapin. ACS Nano 2023, 17, 2, 1315–1326 Surface passivation of intensely luminescent all-inorganic nanocrystals and their direct optical patterning Pengwei Xiao, Zhoufan Zhang, Junjun Ge, Yalei Deng, Xufeng Chen, Jian-Rong Zhang, Zhengtao Deng, Yu Kambe, Dmitri V. Talapin, and Yuanyuan Wang. Nature Commun. 2023, 14, 49 Thermal Stability of Semiconductor Nanocrystal Solids: Understanding Nanocrystal Sintering and Grain Growth W.nyong Liu, Vishwas Srivastava, J. Matthew Kurley, Chengyang Jiang, and Dmitri V. Talapin. Journal of Physical Chemistry C 2022, 126, 39, 21136–21148 Intrinsic glassy-metallic transport in an amorphous coordination polymer Jiaze Xie, Simon Ewing, Jan-Niklas Boyn, Alexander S. Filatov, Baorui Cheng, Tengzhou Ma, Garrett Grocke, Norman Zhao, Ram Itani, Xiaotong Sun, Himchan Cho, Zhihengyu Chen, Karena W. Chapman, Shrayesh N. Patel, Dmitri V. Talapin, Jiwoong Park, David A. Mazziotti, and John S. Anderson. Nature 2022, 611, 479-484 Presynthetic Redox Gated Metal-to-Insulator Transition and Photothermoelectric Properties in Nickel Tetrathiafulvalene-Tetrathiolate Coordination Polymers Jiaze Xie, Jia-Ahn Pan, Baorui Cheng, Tengzhou Ma, Alexander S. Filatov, Shrayesh N. Patel, Jiwoong Park, Dmitri V. Talapin, and John S. Anderson. J. Amer. Chem. Soc. 2022, 144, 41, 19026–19037 Ligand-Free Direct Optical Lithography of Bare Colloidal Nanocrystals via Photo-Oxidation of Surface Ions with Porosity Control Jia-Ahn Pan, Haoqi Wu, Anthony Gomez, Justin C. Ondry, Joshua Portner, Wooje Cho, Alex Hinkle, Di Wang, and Dmitri V. Talapin. ACS Nano 2022, 16, 10, 16067–16076 3D-printing nanocrystals with light (Perspective) Jia-Ahn Pan and Dmitri V. Talapin. Science 2022, 377, 6610, 1046-1047 Diffusion-Limited Kinetics of Isovalent Cation Exchange in III-V Nanocrystals Dispersed in Molten Salt Reaction Media Aritrajit Gupta, Justin Ondry, Min Chen, Margaret H. Hudson, Igor Coropceanu, Nivedina A. Sarma, and Dmitri V. Talapin. Nano Lett. 2022, 22, 16, 6545-6552 Direct Heat-Induced Patterning of Inorganic Nanomaterials Haoqi Wu, Yuanyuan Wang, Jaehyung Yu, Jia-Ahn Pan, Himchan Cho, Aritrajit Gupta, Igor Coropceanu, Chenkun Zhou, Jiwoong Park, and Dmitri V. Talapin. J. Amer. Chem. Soc. 2022, 144, 23, 10495–10506 Self-Assembly of Nanocrystals into Strongly Electronically Coupled All-Inorganic Supercrystals Igor Coropceanu, Eric M. Janke, Joshua Portner, Danny Haubold, Trung Dac Nguyen, Avishek Das, Christian P. N. Tanner, James K. Utterback, Samuel W. Teitelbaum, Margaret H. Hudson, Nivedina A. Sarma, Alex M. Hinkle, Christopher J. Tassone, Alexander Eychmüller, David T. Limmer, Monica Olvera de la Cruz, Naomi S. Ginsberg, and Dmitri V. Talapin. Science 2022, 375, 6587, 1422–1426 Synthesis of In1–xGaxP Quantum Dots in Lewis Basic Molten Salts: The Effects of Surface Chemistry, Reaction Conditions, and Molten Salt Composition M.rgaret H. Hudson, Aritrajit Gupta, Vishwas Srivastava, Eric M. Janke, and Dmitri V. Talapin. J. Phys. Chem. C. 2022, 126, 3, 1564–1580 Active learning of polarizable nanoparticle phase diagrams for the guided design of triggerable self-assembling superlattices Siva Dasetty, Igor Coropceanu, Joshua Portner, Jiyuan Lia, Juan J. de Pablo, Dmitri Talapin, and Andrew L. Ferguson. Mol. Syst. Des. Eng. 2022, 7, 350-363 Magnetoresistance of high mobility HgTe quantum dot films with controlled charging M.nglu Chen, Xinzheng Lan, Margaret H. Hudson, Guohua Shen, Peter B. Littlewood, Dmitri V. Talapin and Philippe Guyot-Sionnest. J. Mater. Chem. C 2022, 10, 13771–13777 Roll-To-Roll Friendly Solution-Processing of Ultrathin, Sintered CdTe Nanocrystal Photovoltaics J. Matthew Kurley,⊥ Jia-Ahn Pan,⊥ Yuanyuan Wang, Hao Zhang, Jake C. Russell, Gregory F. Pach, B.bby To, Joseph M. Luther, and Dmitri V. Talapin. ACS Appl. Mater. Interfaces. 2021, 13, 37, 44165-44173 Direct Optical Lithography of CsPbX3 Nanocrystals via Photoinduced Ligand Cleavage with Postpatterning Chemical Modification and Electronic Coupling Jia-Ahn Pan, Justin C. Ondry, Dmitri V. Talapin. Nano Lett. 2021, 21, 18, 7609-7616 Semiconductor quantum dots: Technological progress and future challenges F. Pelayo García de Arquer, Dmitri V. Talapin, Victor I. Klimov, Yasuhiko Arakawa, Manfred Bayer, Edward H. Sargent. Science 2021, 373, 640, eaaz8541. Advanced Materials for Energy-Water Systems: The Central Role of Water/Solid Interfaces in Adsorption, Reactivity, and Transport E.ward Barry, Raelyn Burns, Wei Chen, Guilhem X De Hoe, Joan Manuel Montes De Oca, Juan J de Pablo, James Dombrowski, Jeffrey W Elam, Alanna M Felts, Giulia Galli, John Hack, Qiming He, Xiang He, Eli Hoenig, Aysenur Iscen, Benjamin Kash, Harold H Kung, Nicholas HC Lewis, Chong Liu, Xinyou Ma, Anil Mane, Alex BF Martinson, Karen L Mulfort, Julia Murphy, Kristian Mølhave, Paul Nealey, Yijun Qiao, Vepa Rozyyev, George C Schatz, Steven J Sibener, Dmitri Talapin, David M Tiede, Matthew V Tirrell, Andrei Tokmakoff, Gregory A Voth, Zhongyang Wang, Zifan Ye, Murat Yesibolati, Nestor J Zaluzec, Seth B Darling. Chem. Rev. 2021, 121, 15, 9450–9501 Observation of biexciton emission from single semiconductor nanoplatelets Lintao Peng, Wooje Cho, Xufeng Zhang, Dmitri Talapin, Xuedan Ma. Phys. Rev. Mat. 2021, 5, 5, L051601. Nanoscale Disorder Generates Subdiffusive Heat Transport in Self-Assembled Nanocrystal Films James K Utterback, Aditya Sood, Igor Coropceanu, Burak Guzelturk, Dmitri V Talapin, Aaron M Lindenberg, Naomi S Ginsberg. Nano Lett. 2021, 21, 8, 3540–3547. Room temperature single-photon superfluorescence from a single epitaxial cuboid nano-heterostructure John P Philbin, Joseph Kelly, Lintao Peng, Igor Coropceanu, Abhijit Hazarika, Dmitri V Talapin, Eran Rabani, Xuedan Ma, Prineha Narang. arXiv. 2021. Dynamic lattice distortions driven by surface trapping in semiconductor nanocrystals B.rak Guzelturk, Benjamin L Cotts, Dipti Jasrasaria, John P Philbin, David A Hanifi, Brent A Koscher, Arunima D Balan, Ethan Curling, Marc Zajac, Suji Park, Nuri Yazdani, Clara Nyby, Vladislav Kamysbayev, Stefan Fischer, Zach Nett, Xiaozhe Shen, Michael E Kozina, Ming-Fu Lin, Alexander H Reid, Stephen P Weathersby, Richard D Schaller, Vanessa Wood, Xijie Wang, Jennifer A Dionne, Dmitri V Talapin, A Paul Alivisatos, Alberto Salleo, Eran Rabani, Aaron M Lindenberg. Nat. Com. 2021, 12, 1. Direct Optical Lithography of Colloidal Metal Oxide Nanomaterials for Diffractive Optical Elements with 2π Phase Control Jia-Ahn Pan, Zichao Rong, Yuanyuan Wang, Himchan Cho, Igor Coropceanu, Haoqi Wu, and Dmitri V. Talapin. J. Am. Chem. Soc. 2021, 143, 5, 2372–2383. Stoichiometry of the Core Determines the Electronic Structure of Core–Shell III–V/II–VI Nanoparticles M.riami Rusishvili, Stefan Wippermann, Dmitri V. Talapin, and Giulia Galli. Chem. Mater. 2020, 32, 9798-9804. Functional materials and devices by self-assembly Dmitri V. Talapin, Michael Engel, and Paul V. Braun. MRS Bull. 2020, 45, 799. Direct Optical Patterning of Quantum Dot Light‐Emitting Diodes via In Situ Ligand Exchange Himchan Cho, Jia‐Ahn Pan, Haoqi Wu, Xinzheng Lan, Igor Coropceanu, Yuanyuan Wang, Wooje Cho, Ethan A. Hill, John S. Anderson, and Dmitri V. Talapin. Adv. Mater. 2020, 32, 2003805. Area and thickness dependence of Auger recombination in nanoplatelets John P. Philbin, Alexandra Brumberg, Benjamin T. Diroll, Wooje Cho, Dmitri V. Talapin, Richard D. Schaller, and Eran Rabani. J. Chem. Phys. 2020, 153, 054104. Covalent surface modifications and superconductivity of two-dimensional metal carbide MXenes V.adislav Kamysbayev, Alexander S. Filatov, Huicheng Hu, Xue Rui, Francisco Lagunas, Di Wang, Robert F. Klie, and Dmitri V. Talapin. Science 2020, 369, 979. sasPDF: pair distribution function analysis of nanoparticle assemblies from small-angle scattering data Chia-Hao Liu, Eric M. Janke, Ruipen Li, Pavol Juhás, Oleg Gang, Dmitri V. Talapin, and Simon J. L. Billinge. J. Appl. Cryst. 2020, 53, 699. Bright trion emission from semiconductor nanoplatelets Lintao Peng, Matthew Otten, Abhijit Hazarika, Igor Coropceanu, Moritz Cygorek, Gary P. Wiederrecht, Pawel Hawrylak, Dmitri V. Talapin, and Xuedan Ma. Phys. Rev. Materials 2020, 4, 056006. Heat-driven acoustic phonons in lamellar nanoplatelet assemblies B.njamin T. Diroll, Vladislav Kamysbayev, Igor Coropceanu, Dmitri V. Talapin, and Richard D. Schaller. Nanoscale 2020, 12, 9661. Nonequilibrium Thermodynamics of Colloidal Gold Nanocrystals Monitored by Ultrafast Electron Diffraction and Optical Scattering Microscopy B.rak Guzelturk, James K. Utterback, Igor Coropceanu, Vladislav Kamysbayev, Eric M. Janke, Marc Zajac, Nuri Yazdani, Benjamin L. Cotts, Suji Park, Aditya Sood, Ming-Fu Lin, Alexander H. Reid, Michael E. Kozina, Xiaozhe Shen, Stephen P. Weathersby, Vanessa Wood, Alberto Salleo, Xijie Wang, Dmitri V. Talapin, Naomi S. Ginsberg, and Aaron M. Lindenberg. ACS Nano 2020, 14, 4792. Quantized Reaction Pathways for Solution Synthesis of Colloidal ZnSe Nanostructures: A Connection between Clusters, Nanowires, and Two-Dimensional Nanoplatelets P. D. Cunningham, Igor Coropceanu, K. Mulloy, W. Cho, D. V. Talapin. ACS Nano 2020, 14, 3847. Quantum dot solids showing state-resolved band-like transport X. Lan, M. Chen, M. H. Hudson, V. Kamysbayev, Y. Wang, P. Guyot-Sionnest, and D. V. Talapin. Nature Mater. 2020, 19, 323. Hot-Carrier Relaxation in CdSe/CdS Core/Shell Nanoplatelets M. Pelton, Y, Wang, I. Fedin, D. V. Talapin, S. K. O’Leary. J. Phys. Chem. C 2020, 124, 1020. Titanium Nitride Modified Photoluminescence from Single Semiconductor Nanoplatelets L. Peng, X. Wang, I. Coropceanu, A. B. Martinson, H. Wang, D. V. Talapin, and X. Ma. Adv. Funct. Mater. 2020, 30, 1904179. Direct Wavelength-Selective Optical and Electron-Beam Lithography of Functional Inorganic Nanomaterials Y. Wang, J.-A. Pan, H. Wu, and D. V. Talapin. ACS Nano 2019, 13, 13917. Colloidal Gelation in Liquid Metals Enables Functional Nanocomposites of 2D Metal Carbides (MXenes) and Lightweight Metals V. Kamysbayev, N. M. James, A. S. Filatov, V. Srivastava, B. Anasori, H. M. Jaeger, Y. Gogotsi, and D. V. Talapin. ACS Nano 2019, 13, 12415. Polarized near-infrared intersubband absorptions in CdSe colloidal quantum wells B. T. Diroll, M. Chen, I. Coropceanu, K. R. Williams, D. V. Talapin, P. Guyot-Sionnest, and R. D. Schaller. Nat. Commun. 2019, 10, 4511. High Carrier Mobility in HgTe Quantum Dot Solids Improves Mid-IR Photodetectors M. Chen, X. Lan, X. Tang, Y. Wang, M. H. Hudson, D. V. Talapin, and P. Guyot-Sionnest. ACS Photonics 2019, 6, 2358. Colloidal Atomic Layer Deposition with Stationary Reactant Phases Enables Precise Synthesis of “Digital” II-VI Nano-heterostructures with Exquisite Control of Confinement and Strain A. Hazarika, I. Fedin, L. Hong, J. Guo, V. Srivastava, W. Cho, I. Coropceanu, J. C. Portner, B. T. Diroll, J. P. Philbin, E. Rabani, R. F. Klie, and D. V. Talapin. J. Am. Chem. Soc. 2019, 141, 13487. Uniaxial transition dipole moments in semiconductor quantum rings caused by broken rotational symmetry N. F. Hartmann, M. Otten, I. Fedin, D. V. Talapin, M. Cygorek, P. Hawrylak, M. Korkusinski, S. Gray, A. Hartschuh, and X. Ma. Nat. Commun. 2019, 10, 3253. Binary Assembly of PbS and Au Nanocrystals: Patchy PbS Surface Ligand Coverage Stabilizes the CuAu Superlattice M. Boles and D. V. Talapin. ACS Nano 2019, 13, 5375. Nanocrystals in Molten Salts and Ionic Liquids: Experimental Observation of Ionic Correlations Extending beyond the Debye Length V. Kamysbayev, V. Srivastava, N. B. Ludwig, O. J. Borkiewicz, H. Zhang, J. Ilavsky, B. Lee, K. W. Chapman, S. Vaikuntanathan, D. V. Talapin. ACS Nano 2019, 13, 5760. Systematic Mapping of Binary Nanocrystal Superlattices: The Role of Topology in Phase Selection I. Coropceanu, M. A. Boles, D. V. Talapin. J. Am. Chem. Soc. 2019, 141, 5728. Describing screening in dense ionic liquids with a charge-frustrated Ising model N. B. Ludwig, K. Dasbiswas, D. V. Talapin, S. Vaikuntanathan. J. Chem. Phys. 2018, 149, 164505. Origin of Broad Emission Spectra in InP Quantum Dots: Contributions from Structural and Electronic Disorder E. M. Janke, N. E. Williams, C. She, D. Zherebetskyy, M. Hudson, L. Wang, D. J. Gosztola, R. D. Schaller, B. Lee, C. Sun, G. S. Engel, D. V. Talapin. J. Am. Chem. Soc. 2018, 140, 15791. Direct Synthesis of Six-Monolayer (1.9 nm) Thick Zinc-Blende CdSe Nanoplatelets Emitting at 585 nm W. Cho, S. Kim, I. Coropceanu, V. Srivastava, B. T. Diroll, A. Hazarika, I. Fedin, R. D. Schaller, G. Galli, D. V. Talapin. Chem. Mater. 2018, 30, 6957. Semiconductor Nanoplatelet Excimers B. T. Diroll, W. Cho, I. Coropceanu, S. Harvey, A. Brumberg, N. Holtgrewe, S. A. Crooker, M. R. Wasielewski, V. B. Prakapenka, D. V. Talapin, R. D. Schaller. Nano Lett. 2018, 18, 6948. Colloidal Chemistry in Molten Salts: Synthesis of Luminescent In1–xGaxP and In1–xGaxAs Quantum Dots V. Srivastava, V. Kamysbayev, L. Hong, E. Dunietz, R. F. Klie, D. V. Talapin. J. Am. Chem. Soc. 2018, 140, 12144. Conduction Band Fine Structure in Colloidal HgTe Quantum Dots M. H. Hudson, M. Chen, V. Kamysbayev, E. M. Janke, X. Lan, G. Allan, C. Delerue, B. Lee, P. Guyot-Sionnest, D. V. Talapin. ACS Nano 2018, 12, 9397. Anisotropic photoluminescence from isotropic optical transition dipoles in semiconductor nanoplatelets X. Ma, B. T. Diroll, W. Cho, I. Fedin, R. D. Schaller, D. V. Talapin, and G. P. Wiederrecht. Nano Lett. 2018, 18, 4647. Surface chemistry and buried interfaces in all-inorganic nanocrystalline solids E. Scalise, V. Srivastava, E. M. Janke, D. Talapin, G. Galli, and S. Wippermann. Nature Nanotech. 2018, 33, 841. Monodisperse InAs Quantum Dots from Aminoarsine Precursors: Understanding the Role of Reducing Agent V. Srivastava, E. Dunietz, V. Kamysbayev, J. S. Anderson, and D. V. Talapin. Chem. Mater. 2018, 30, 3623. Elevated Temperature Photophysical Properties and Morphological Stability of CdSe and CdSe/CdS Nanoplatelets C. E. Rowland, I. Fedin, B. T. Diroll, Y. Liu, D. V. Talapin, and R. D. Schaller. J. Phys. Chem. Lett. 2018, 9, 286.

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