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Bowen Li§, Jianzhong Chen§, Wanbin Zhang*, Efficient Preparation of ChiralHydroxylamines via Nickel-Catalyzed Asymmetric Hydrogenation of Oximes. Org. Synth. 2025, 102, 236-250. DOI: 10.15227/orgsyn.102.0236.
Zijiao Liu§, Panpan Li§, Haoyang Wang, Jiacheng Zhang, Xiaohong Huo*, Zhen-Liang Sun,* Wanbin Zhang*, Ternary Aldehyde-Copper-Iridium Catalysis Enables Stereodivergent Allylation via α-C-H Functionalization of Primary Amines. Angew. Chem. Int. Ed. 2025, 64, e202508335. DOI: 10.1002/anie.202508335.
Yuxi Song, Yashi Zou, Tiantian Chen, Zhenfeng Zhang*, Wanbin Zhang*, Cobalt-Catalyzed Asymmetric Hydrogenation of -Hydroxy Ketones Enabled by a Carboxylic Acid Additive Promotion Strategy, Angew. Chem. Int. Ed. 2025, 64, e202504159. DOI: 10.1002/anie.202504159.
Jianzhong Chen, Hanlin Wei, Ilya D. Gridnev, and Wanbin Zhang*, Weak Attractive Noncovalent Interactions in Metal-Catalyzed Asymmetric Hydrogenation, Angew. Chem. Int. Ed. 2025, 64, e202425589. DOI: 10.1002/anie.202425589.
Hanlin Wei, Yicong Luo, Jinhui Li, Jianzhong Chen,* Ilya D. Gridnev,* and Wanbin Zhang*, Enantioselective Synthesis of Chiral β2-Amino Phosphorus Derivatives via Nickel-Catalyzed Asymmetric Hydrogenation. J. Am. Chem. Soc. 2025, 147, 342-352. DOI: 10.1021/jacs.4c10623.
Jing Guan, Yicong Luo, Qiyuan Wang, Jianzhong Chen*, Wanbin Zhang*, Copper-Catalyzed Asymmetric Hydrogenation of Unsymmetrical ortho-Br Substituted Benzophenones, Angew. Chem. Int. Ed. 2025, 64, e202416313. DOI: 10.1002/anie.202416313.
Haipeng Wei, Yicong Luo, Jinbao Ren, Qianjia Yuan*, Wanbin Zhang*, Ni(II)-catalyzed asymmetric alkenylation and arylation of aryl ketones with organoborons via 1,5-metalate shift”, Nat. Commun. 2024, 15, 8775. DOI: 10.1038/s41467-024-53005-x.
Panpan Li, En Zheng, Guanlin Li, Yicong Luo, Xiaohong Huo, Shengming Ma,* and Wanbin Zhang*, Stereodivergent access to non-natural α-amino acids via enantio- and Z/E-selective catalysis, Science 2024, 385, 972-979. DOI: 10.1126/science.ado4936.
Zhengdong Ding, Yicong Luo, Qianjia Yuan, Guangjie Wang, Zhenpeng Yu, Min Zhao, Delong Liu, and Wanbin Zhang*, Ru-Catalyzed Asymmetric Hydrogenation of α,β-Unsaturated γ-Lactams, J. Am. Chem. Soc. 2024, 146, accepted. DOI: 10.1021/jacs.4c09794.
Wenzhi Zhu, Chongyu Han, Guoqiang Yang, Xiaohong Huo*, and Wanbin Zhang*, Pd/Cu-Cocatalyzed Enantio- and Diastereodivergent Wacker-Type Dicarbofunctionalization of Unactivated Alkenes. J. Am. Chem. Soc. 2024, 146, accepted. DOI: 10.1021/jacs.4c06788.
Jiacheng Zhang, Yicong Luo, En Zheng, Xiaohong Huo, Shengming Ma*, and Wanbin Zhang*, Synergistic Pd/Cu-Catalyzed 1,5-Double Chiral Inductions. J. Am. Chem. Soc. 2024, 146, 9241–9251. DOI: 10.1021/jacs.4c00497.
Bowen Li, Zhiling Wang, Yicong Luo, Hanlin Wei, Jianzhong Chen,* Delong Liu, and Wanbin Zhang*, Nickel-Catalyzed Asymmetric Hydrogenation for the Preparation of α-Substituted Propionic Acids. Nat. Commun. 2024, 15, 5482. DOI: doi.org/10.1038/s41467-024-49801-0.
Panpan Li, Zijiao Liu, Xiaohong Huo*, and Wanbin Zhang*, Stereodivergent Construction of 1,5/1,7-Nonadjacent Tetrasubstituted Stereocenters Enabled by Pd/Cu-Cocatalyzed Asymmetric Heck Cascade Reaction. Angew. Chem. Int. Ed. 2024, 63, e202407498. DOI: 10.1002/anie.202407498.
Youbin Peng, Guanlin Li, Chongyu Han, Yicong Luo, Xiaohong Huo*, and Wanbin Zhang*, Stereodivergent Benzylic Substitution of Racemic Secondary Benzyl Esters Enabled by Pd/Cu Dual Catalysis. CCS Chem. 2024, accepted. DOI: 10.31635/ccschem.024.202303749.
Huiwen Yang, Yanhua Hu, Yashi Zou, Zhenfeng Zhang,* and Wanbin Zhang*. Cobalt-Catalyzed Efficient Asymmetric Hydrogenation of α-Primary Amino Ketones, JACS Au 2023, accepted. DOI: 10.1021/jacsau.3c00524.
Yicong Luo, Yuqi Ma, Guanlin Li, Xiaohong Huo,* and Wanbin Zhang*. Desymmetrization of Geminal Difluoromethylenes using a Palladium/Copper/Lithium Ternary System for the Stereodivergent Synthesis of Fluorinated Amino Acids, Angew. Chem. Int. Ed. 2023, 62, e202313838. DOI: 10.1002/anie.202313838.
Fei Li, Yicong Luo, Jinbao Ren, Qianjia Yuan,* Deyue Yan, and Wanbin Zhang*. Iridium-Catalyzed Remote Site-Switchable Hydroarylation of Alkenes Controlled by Ligands, Angew. Chem. Int. Ed. 2023, 62, e202309859. DOI: 10.1002/anie.202309859.
Yunnan Xu, Yicong Luo, Jianxun Ye, Delong Liu, and Wanbin Zhang*. Rh-Catalyzed Enantioselective Desymmetric Hydrogenation of α-Acetamido-1,3-indanediones Using Ether-Bridged Biphenyl Diphosphine Ligands. J. Am. Chem. Soc. 2023, 145, 21176-21182. DOI: 10.1021/jacs.3c07509.
Jing Guan, Jianzhong Chen, Yicong Luo, Lisen Guo, and Wanbin Zhang*, Copper-Catalyzed Chemoselective Asymmetric Hydrogenation of C=O Bonds of Exocyclic α,β-Unsaturated Pentanones. Angew. Chem. Int. Ed. 2023, 62, e202306380. DOI: 10.1002/anie.202306380.
Cheng Sheng, Zheng Ling, Junzhe Xiao, Kai Yang, Fang Xie, Shengming Ma*, and Wanbin Zhang*, Enantio- and Diastereoselective Synthesis of Chiral Tetrasubstituted α-Amino Allenoates Bearing a Vicinal All-Carbon Quaternary Stereocenter with Dual-Copper-Catalysis. Angew. Chem. Int. Ed. 2023, 62, e202305680. DOI: 10.1002/anie.202305680.
Zhengxing Wu, Jingjie Meng, Huikang Liu, Yunyi Li, Xiao Zhang, and Wanbin Zhang*, Multisite programmable functionalization of alkenes via controllable alkene isomerization. Nat. Chem. 2023, 15, 988-997. DOI: 10.1038/s41557-023-01209-x.
Liang Tang, Yicong Luo, Cheng Sheng, Fang Xie*, and Wanbin Zhang*, Cu-Catalyzed Asymmetric Kinetic Boron Conjugate Addition of γ-Substituted α,β-Unsaturated γ-Lactams. Angew. Chem. Int. Ed. 2023, 62, e202304640. DOI: 10.1002/anie.202304640.
Tiantian Chen, Yashi Zou, Yanhua Hu, Zhenfeng Zhang, Hao Wei, Liangming Wei, and Wanbin Zhang*, Cobalt-Catalyzed Efficient Convergent Asymmetric Hydrogenation of E/Z-Enamides. Angew. Chem. Int. Ed. 2023, 62, e202303488. DOI: 10.1002/anie.202303488.
Yanhua Hu, Yashi Zou, Huiwen Yang, Haotian Ji, Yue Jin, Zhenfeng Zhang,* Yangang Liu, and Wanbin Zhang*, Precise Synthesis of Chiral Z-Allylamides by Cobalt-Catalyzed Asymmetric Sequential Hydrogenations. Angew. Chem. Int. Ed. 2023, 62, e202217871. DOI: 10.1002/anie.202217871.
Ling Zhao, Yicong Luo, Junzhe Xiao, Xiaohong Huo, Shengming Ma,* and Wanbin Zhang*, Stereodivergent Synthesis of Allenes with α,β-Adjacent Central Chiralities Empowered by Synergistic Pd/Cu Catalysis. Angew. Chem. Int. Ed. 2023, 62, e202218146. DOI: 10.1002/anie.202218146.
Hanlin Wei, Hao Chen, Jianzhong Chen*, Ilya. D. Gridnev,* and Wanbin Zhang*, Nickel-Catalyzed Asymmetric Hydrogenation of α-Substituted Vinylphosphonates and Diarylvinylphosphine Oxides. Angew. Chem. Int. Ed. 2023, 62, e202214990. DOI: 10.1002/anie.202214990.
Yunnan Xu, Yicong Luo, Jianxun Ye, Yu Deng, Delong Liu, and Wanbin Zhang*, Rh-Catalyzed Sequential Asymmetric Hydrogenations of 3-Amino-4-Chromones via an Unusual Dynamic Kinetic Resolution Process. J. Am. Chem. Soc. 2022, 144, 20078-20089. DOI: 10.1021/jacs.2c09266
Feng Gao, Jing Li, Tanveer Ahmad, Yicong Luo, Zhenfeng Zhang, Qianjia Yuan, Xiaohong Huo, Tao Song, and Wanbin Zhang*, Sci. China Chem. 2022, 65, 1968-1977. DOI: 10.1007/s11426-022-1387-7.
Mo Wang,§ Zhenfeng Zhang,§ and Wanbin Zhang*, Design, Synthesis and Application of Chiral Bicyclic Imidazole Catalysts. Acc. Chem. Res. 2022, 55, 2708-2727. DOI: 10.1021/acs.accounts.2c00455.
Xiaohong Huo, Guanlin Li, Xi Wang, and Wanbin Zhang*, Bimetallic Catalysis in Stereodivergent Synthesis. Angew. Chem. Int. Ed. 2022, 61, e202210086. DOI: 10.1002/anie.202210086.
Biwen Li, Jianzhong Chen, Dan Liu, Ilya D. Gridnev, and Wanbin Zhang*, Nickel-catalysed asymmetric hydrogenation of oximes. Nat. Chem. 2022, 14, 920-927. DOI: 10.1038/s41557-022-00971-8.
Youbin Peng, Chongyu Han, Yicong Luo, Guanlin Li, XiaohongHuo, and Wanbin Zhang*, Nickel/Copper-Cocatalyzed Asymmetric Benzylation of Aldimine Esters for the Enantioselective Synthesis of α-Quaternary Amino Acids. Angew. Chem. Int. Ed. 2022, 61, e202203448. DOI: 10.1002/anie.202203448.
Muxing Zhou, Yashi Zou, Lu Zhang, Zhenfeng Zhang, and Wanbin Zhang*, Chiral Bicyclic Imidazole-Catalyzed Direct Enantioselective C-Acetylation of Indolones. CCS Chem. 2022, 5, 361-371. DOI: 10.31635/ccschem.022.202201782.
Cheng Sheng, Zheng Ling, Yicong Luo, and Wanbin Zhang*, Cu-catalyzed asymmetric addition of alcohols to β,γ-alkynyl-α-imino esters for the construction of linear chiral N,O-ketals. Nat. Commun. 2022, 13, 400. DOI: 10.1038/s41467-022-28002-7.
Youbin Peng, Xiaohong Huo, Yicong Luo, Liang Wu, and Wanbin Zhang*, Enantio- and Diastereodivergent Synthesis of Spirocycles through Dual-Metal-Catalyzed [3+2] Annulation of 2-Vinyloxiranes with Nucleophilic Dipoles. Angew. Chem. Int. Ed. 2021, 60, 24941-24949. DOI: 10.1002/anie.202111842.
Yunnan Xu, Delong Liu, Yu Deng, Yi Zhou, and Wanbin Zhang*, Rh-Catalyzed Asymmetric Hydrogenation of 3-Benzoylaminocoumarins for the Synthesis of Chiral 3-Amino Dihydrocoumarins. Angew. Chem. Int. Ed. 2021, 60, 23602-23607. DOI: 10.1002/anie.202110286.
Jiacheng Zhang, Xiaohong Huo, Junzhe Xiao, Ling Zhao, Shengming Ma*, and Wanbin Zhang*, Enantio- and Diastereodivergent Construction of 1,3-Nonadjacent Stereocenters Bearing Axial and Central Chirality through Synergistic Pd/Cu Catalysis. J. Am. Chem. Soc. 2021, 143, 12622-12632. DOI: 10.1021/jacs.1c05087.
Jian Zhang, Tiantian Chen, Yuanhao Wang, Fengfan Zhou, Zhenfeng Zhang*, Ilya D. Gridnev*, and Wanbin Zhang*, Asymmetric Hydrogenation of γ-Branched Allylamines for the Efficient Synthesis of γ-Chirogenic Amines. Nat. Sci. 2021, e10021. DOI: 10.1002/ntls.10021.
Yanhua Hu, Zhenfeng Zhang, Yangang Liu, and Wanbin Zhang*, Cobalt-Catalyzed Chemo- and Enantioselective Hydrogenation of Conjugated Enynes. Angew. Chem. Int. Ed. 2021, 60, 16989-16993. DOI: 10.1002/anie.202106566.
Xiaohong Huo, Ling Zhao, Yicong Luo, Yue Wu, Yuwen Sun, Guanlin Li, Tatiana Gridneva, Jiacheng Zhang, Yong Ye, and Wanbin Zhang*, Stereodivergent Pd/Cu Catalysis for Asymmetric Desymmetric Alkylation of Allylic Geminal Dicarboxylates. CCS Chem. 2021, 3, 1933-1944. DOI: 10.31635/ccschem.021.202101044.
Chong Liu, Jing Yuan, Zhenfeng Zhang*, Ilya D. Gridnev, and Wanbin Zhang*, Asymmetric Hydroacylation Involving Alkene Isomerization for the Construction of C3-Chirogenic Center. Angew. Chem. Int. Ed. 2021, 60(16), 8997-9002. DOI: 10.1002/anie.202017190
Muxing Zhou, Tatiana Gridneva, Zhenfeng Zhang, Ende He, Yangang Liu, and Wanbin Zhang*, Chiral Bicyclic Imidazole-Catalyzed Acylative Dynamic Kinetic Resolution for the Synthesis of Chiral Phthalidyl Esters. Angew. Chem. Int. Ed. 2021, 60(3), 1641-1645. DOI: 10.1002/anie.202012445
Dan Liu, Bowen Li, Jianzhong Chen, Ilya D. Gridnev, Deyue Yan, and Wanbin Zhang*, Ni-Catalyzed Asymmetric Hydrogenation of N-Aryl Imino Esters for the Efficient Synthesis of Chiral α-Aryl Glycines. Nat. Commun. 2020, 11, 5935. DOI: 10.1038/s41467-020-19807-5
Mo Wang, Lu Zhang, Xiaohong Huo, Zhenfeng Zhang, Qianjia Yuan, Panpan Li, Jianzhong Chen, Yashi Zou, Zhengxing Wu, and Wanbin Zhang*, Catalytic Asymmetric Synthesis of the anti-COVID-19 Drug Remdesivir. Angew. Chem. Int. Ed. 2020, 59(47), 20814-20819. DOI: 10.1002/anie.202011527
Rui He, Xiaohong Huo, Ling Zhao, Feijun Wang, Liyin Jiang, Jian Liao*, and Wanbin Zhang*, Stereodivergent Pd/Cu Catalysis for the Dynamic Kinetic Asymmetric Transformation of Racemic Unsymmetrical 1,3-Disubstituted Allyl Acetates. J. Am. Chem. Soc. 2020, 142(18), 8097-8103.
Guanlin Li, Xiaohong Huo, Xieyang Jiang, and Wanbin Zhang*, Asymmetric Synthesis of Allylic Compounds via Hydrofunctionalisation and Difunctionalisation of Dienes, Allenes, and Alkynes. Chem. Soc. Rev. 2020, 49(7), 2060-2118. DOI: 10.1039/c9cs00400a
Yawen Hu, Jianzhong Chen, Bowen Li, Zhenfeng Zhang, Ilya D. Gridnev, and Wanbin Zhang*, Nickel-Catalyzed Asymmetric Hydrogenation of 2-Amidoacrylates. Angew. Chem. Int. Ed. 2020, 59(13), 5371-5375. DOI: 10.1002/anie.201916534
Liang Wu, Guoqiang Yang, and Wanbin Zhang*, Ni-Catalyzed Enantioconvergent Coupling of Epoxides with Alkenylboronic Acids: Construction of Oxindoles Bearing Quaternary Carbons. CCS Chem. 2020, 2(2), 623-631. DOI: 10.31635/ccschem.019.201900064
Yanhua Hu, Zhenfeng Zhang, Jian Zhang, Yangang Liu, Ilya D. Gridnev, and Wanbin Zhang*, Cobalt-Catalyzed Asymmetric Hydrogenation of C=N Bonds Enabled by Assisted Coordination and Nonbonding Interactions. Angew. Chem. Int. Ed. 2019, 58(44), 15767-15771. DOI: 10.1002/anie.201909928
Jian Zhang, Jia Jia, Xincheng Zeng, Yuanhao Wang, Zhenfeng Zhang, Ilya D. Gridnev, and Wanbin Zhang*, Chemo- and Enantioselective Hydrogenation of α-Formyl Enamides: An Efficient Access to Chiral α-Amido Aldehydes. Angew. Chem. Int. Ed. 2019, 58(33), 11505-11512. DOI: 10.1002/anie.201905263
Bowen Li, Jianzhong Chen, Zhenfeng Zhang, Ilya D. Gridnev, and Wanbin Zhang*, Nickel-Catalyzed Asymmetric Hydrogenation of N-Sulfonyl Imines. Angew. Chem. Int. Ed. 2019, 58(22), 7329-7334. DOI: 10.1002/anie.201902576
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